Surface Modification of Diamond-Like Carbon Film with Polymer Brushes Using a Bio-Inspired Catechol Anchor for Excellent Biological Lubrication
文献类型：期刊论文
| 作者 | Wei QB(魏强兵) ; Pei XW(裴小维); Hao JY(郝俊英); Cai MR(蔡美荣); Zhou F(周峰); Liu WM(刘维民); Cai MR(蔡美荣); Zhou F(周峰); Cai MR(蔡美荣); Cai MR(蔡美荣)
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| 刊名 | Advanced Materials Interfaces
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| 出版日期 | 2014 |
| 卷号 | 1页码:1400035(1-8) |
| ISSN号 | 2196-7350 |
| 通讯作者 | 蔡美荣 ; 周峰 |
| 英文摘要 | Diamond-like carbon (DLC) film has emerged as a promising material for biomedical applications, but its low tribological properties in air could not be adapted in water and biological fluids. Herein, mussel-inspired catechol adhesive is presented to functionalize DLC film and then polymer brushes are grafted by surface initiated atom transfer radical polymerization (SI-ATRP) to mimic excellent biological lubrication of articular cartilage. Macroscopic tribological evaluation demonstrates low and stable friction coefficient of polymer brushe modified DLC film in water and biological fluids when sliding with a soft polydimethylsiloxane (PDMS) hemisphere, owing to viscous fluid-like boundary lubricant film being formed by high hydration of polymer chains. The strong adhesive capability of catechol anchors also prevents polymer chains being sheared off from the substrate during friction tests. The friction responsiveness of PSPMA brushes is observed in electrolyte solution due to the conformation change of polymer chains. The successful functionalization of DLC with polymer brushes affords DLC film excellent biological lubrication and thus will broaden the scope of its applications in biomedical field. |
| 学科主题 | 材料科学与物理化学 |
| 资助信息 | NSFC (21125316;51305428;51335010);the Key Research Program of the Chinese Academy of Sciences (grant no., KJZD-EW-M01);the “973” project of the Chinese Ministry of Science and Technology (2013CB632300) |
| 语种 | 英语 |
| WOS记录号 | WOS:000348283700013 |
| 公开日期 | 2014-12-05 |
| 源URL | [http://210.77.64.217/handle/362003/6862]  |
| 专题 | 兰州化学物理研究所_固体润滑国家重点实验室 |
| 通讯作者 | Cai MR(蔡美荣); Zhou F(周峰); Cai MR(蔡美荣); Cai MR(蔡美荣); Cai MR(蔡美荣); Cai MR(蔡美荣); Cai MR(蔡美荣) |
| 推荐引用方式 GB/T 7714 | Wei QB,Pei XW,Hao JY,et al. Surface Modification of Diamond-Like Carbon Film with Polymer Brushes Using a Bio-Inspired Catechol Anchor for Excellent Biological Lubrication[J]. Advanced Materials Interfaces,2014,1:1400035(1-8). |
| APA | Wei QB.,Pei XW.,Hao JY.,Cai MR.,Zhou F.,...&蔡美荣.(2014).Surface Modification of Diamond-Like Carbon Film with Polymer Brushes Using a Bio-Inspired Catechol Anchor for Excellent Biological Lubrication.Advanced Materials Interfaces,1,1400035(1-8). |
| MLA | Wei QB,et al."Surface Modification of Diamond-Like Carbon Film with Polymer Brushes Using a Bio-Inspired Catechol Anchor for Excellent Biological Lubrication".Advanced Materials Interfaces 1(2014):1400035(1-8). |
入库方式： OAI收割
来源：兰州化学物理研究所
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