Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions
文献类型:期刊论文
作者 | Jiang, BJ ; Song, SZ ; Wang, JQ ; Xie, Y ; Chu, WY ; Li, HF ; Xu, H ; Tian, CG ; Fu, HG |
刊名 | NANO RESEARCH
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出版日期 | 2014 |
卷号 | 7期号:9页码:1280—1290 |
关键词 | ENHANCED PHOTOCATALYTIC ACTIVITY RAY-ABSORPTION SPECTROSCOPY PALLADIUM NANOPARTICLES GRAPHITE OXIDE CATALYST FABRICATION REDUCTION RESONANCE FACETS GROWTH |
ISSN号 | 1998-0124 |
通讯作者 | fuhg@vip.sina.com |
英文摘要 | The introduction of nitrogen significantly decreases the metal particle size and improves the performance of metal-based graphene-supported catalysts. In this work, the density functional theory is used to understand the interaction between nitrogen-doped graphene and Pd@PdO clusters. Experiments show that small size Pd@PdO clusters (1-2 nm) can be grown uniformly on nitrogen-doped graphene sheets by a facile oxidation-reduction method. The nanoscale interaction relationship between nitrogen-doped graphene and Pd@PdO clusters is investigated through X-ray photoelectron spectroscopy (XPS) and X-ray absorption spectra (XAS). The composite catalysts are applied in Suzuki-Miyaura reactions giving high yields and good structural stability. These results have potential impact in design and optimization of future high performance catalyst materials for cross coupling reactions. |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000342080100005 |
公开日期 | 2015-03-13 |
源URL | [http://ir.sinap.ac.cn/handle/331007/14274] ![]() |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
推荐引用方式 GB/T 7714 | Jiang, BJ,Song, SZ,Wang, JQ,et al. Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions[J]. NANO RESEARCH,2014,7(9):1280—1290. |
APA | Jiang, BJ.,Song, SZ.,Wang, JQ.,Xie, Y.,Chu, WY.,...&Fu, HG.(2014).Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions.NANO RESEARCH,7(9),1280—1290. |
MLA | Jiang, BJ,et al."Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions".NANO RESEARCH 7.9(2014):1280—1290. |
入库方式: OAI收割
来源:上海应用物理研究所
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