Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method
文献类型:期刊论文
作者 | Wang, Zhen1; Shen, Genli2,3; Li, Jiaqi2,3; Liu, Haidi2; Wang, Qi1; Chen, Yunfa2![]() |
刊名 | APPLIED CATALYSIS B-ENVIRONMENTAL
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出版日期 | 2013-07-17 |
卷号 | 138期号:0页码:253-259 |
关键词 | CeO2-MnOx composite oxides Oxygen vacancy Synergistic effect Benzene oxidation |
英文摘要 | A series of CeO2-MnOx composite oxides were synthesized through hydrothermal method and the complete catalytic oxidation of benzene were examined. The effects of the Ce-at/Mn-at atomic ratio on the features of catalyst structure and catalytic behavior were researched. The results exhibited that the catalytic properties of CeO2-MnOx composite oxides were higher than pure CeO2 or MnOx. When the Ceat/Mnat ratio was 3:7, the catalytic activity reached the best. By means of testing, the data revealed that the synergistic effects existed in the composite oxides, which resulted in the enhancement of catalytic abilities. In the main phase, MnOx provided available oxygen species and CeO2 enhanced oxygen mobility. In addition, the nature of oxygen vacancy of catalysts was also studied through positron annihilation spectrum. The results showed that the concentration of oxygen vacancy for CeO2-MnOx composite oxides changed comparing with pure CeO2 or MnOx, which also caused the activity differences over benzene. (C) 2013 Elsevier B.V. All rights reserved. |
WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
类目[WOS] | Chemistry, Physical ; Engineering, Environmental ; Engineering, Chemical |
研究领域[WOS] | Chemistry ; Engineering |
关键词[WOS] | VOLATILE ORGANIC-COMPOUNDS ; COMPLETE OXIDATION ; LOW-TEMPERATURES ; WET OXIDATION ; CO OXIDATION ; CERIUM OXIDE ; O-XYLENE ; COMBUSTION ; PALLADIUM ; TOLUENE |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000319087900030 |
公开日期 | 2015-05-27 |
源URL | [http://ir.ipe.ac.cn/handle/122111/13558] ![]() |
专题 | 过程工程研究所_研究所(批量导入) |
作者单位 | 1.Natl Ctr Nanosci & Technol, CAS Key Lab Standardizat & Measurement Nanotechno, Beijing 100190, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 3.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Zhen,Shen, Genli,Li, Jiaqi,et al. Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method[J]. APPLIED CATALYSIS B-ENVIRONMENTAL,2013,138(0):253-259. |
APA | Wang, Zhen,Shen, Genli,Li, Jiaqi,Liu, Haidi,Wang, Qi,&Chen, Yunfa.(2013).Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method.APPLIED CATALYSIS B-ENVIRONMENTAL,138(0),253-259. |
MLA | Wang, Zhen,et al."Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method".APPLIED CATALYSIS B-ENVIRONMENTAL 138.0(2013):253-259. |
入库方式: OAI收割
来源:过程工程研究所
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