中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method

文献类型:期刊论文

作者Wang, Zhen1; Shen, Genli2,3; Li, Jiaqi2,3; Liu, Haidi2; Wang, Qi1; Chen, Yunfa2
刊名APPLIED CATALYSIS B-ENVIRONMENTAL
出版日期2013-07-17
卷号138期号:0页码:253-259
关键词CeO2-MnOx composite oxides Oxygen vacancy Synergistic effect Benzene oxidation
英文摘要A series of CeO2-MnOx composite oxides were synthesized through hydrothermal method and the complete catalytic oxidation of benzene were examined. The effects of the Ce-at/Mn-at atomic ratio on the features of catalyst structure and catalytic behavior were researched. The results exhibited that the catalytic properties of CeO2-MnOx composite oxides were higher than pure CeO2 or MnOx. When the Ceat/Mnat ratio was 3:7, the catalytic activity reached the best. By means of testing, the data revealed that the synergistic effects existed in the composite oxides, which resulted in the enhancement of catalytic abilities. In the main phase, MnOx provided available oxygen species and CeO2 enhanced oxygen mobility. In addition, the nature of oxygen vacancy of catalysts was also studied through positron annihilation spectrum. The results showed that the concentration of oxygen vacancy for CeO2-MnOx composite oxides changed comparing with pure CeO2 or MnOx, which also caused the activity differences over benzene. (C) 2013 Elsevier B.V. All rights reserved.
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Physical ; Engineering, Environmental ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]VOLATILE ORGANIC-COMPOUNDS ; COMPLETE OXIDATION ; LOW-TEMPERATURES ; WET OXIDATION ; CO OXIDATION ; CERIUM OXIDE ; O-XYLENE ; COMBUSTION ; PALLADIUM ; TOLUENE
收录类别SCI
语种英语
WOS记录号WOS:000319087900030
公开日期2015-05-27
源URL[http://ir.ipe.ac.cn/handle/122111/13558]  
专题过程工程研究所_研究所(批量导入)
作者单位1.Natl Ctr Nanosci & Technol, CAS Key Lab Standardizat & Measurement Nanotechno, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
3.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Wang, Zhen,Shen, Genli,Li, Jiaqi,et al. Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method[J]. APPLIED CATALYSIS B-ENVIRONMENTAL,2013,138(0):253-259.
APA Wang, Zhen,Shen, Genli,Li, Jiaqi,Liu, Haidi,Wang, Qi,&Chen, Yunfa.(2013).Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method.APPLIED CATALYSIS B-ENVIRONMENTAL,138(0),253-259.
MLA Wang, Zhen,et al."Catalytic removal of benzene over CeO2-MnOx composite oxides prepared by hydrothermal method".APPLIED CATALYSIS B-ENVIRONMENTAL 138.0(2013):253-259.

入库方式: OAI收割

来源:过程工程研究所

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