Enhanced fluidized bed methanation over a Ni/Al2O3 catalyst for production of synthetic natural gas
文献类型：期刊论文
| 作者 | Li, Jun1; Zhou, Li1; Li, Pengcheng1,2; Zhu, Qingshan1; Gao, Jiajian1,2; Gu, Fangna1; Su, Fabing1 |
| 刊名 | CHEMICAL ENGINEERING JOURNAL
 |
| 出版日期 | 2013-03-01 |
| 卷号 | 219期号:0页码:183-189 |
| 关键词 | CO methanation Fluidized bed Synthetic natural gas |
| 英文摘要 | The fluidization behavior and CO methanation performance over a typical Ni/Al2O3 catalyst for synthetic natural gas production was systematically investigated in a fluidized bed reactor. The results indicated that the methanation performance of the catalyst depends, to a large extent, on the fluidization quality in the fluidized-bed methanation reactor. The pure Ni/Al2O3 catalyst with the particle sizes of 10-100 mu m failed to fluid, but the fluidization can be significantly improved by adding Al2O3 particles. The methanation reaction in the fluidized bed reactor was also substantially improved by adding Al2O3 particles, and the yield and selectivity of CH4 in the fluidized bed with Al2O3 addition were much higher than those of without Al2O3 addition. The CO methanation reaction was controlled by two different mechanisms, i.e. the surface reaction controlling in lower temperature range (250-330 degrees C) and external diffusion controlling in higher temperature range (>330 degrees C). Stability test demonstrated that the fluidized bed methanation reactor showed higher CO conversion, CH4 selectivity and yield, and more excellent carbon resistance than the fixed bed methanation reactor under high temperature, which is beneficial for reclaiming the high temperature steam. (C) 2013 Elsevier B.V. All rights reserved. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Engineering, Environmental ; Engineering, Chemical |
| 研究领域[WOS] | Engineering |
| 关键词[WOS] | SELECTIVE METHANATION ; MICROCHANNEL REACTOR ; COHESIVE PARTICLES ; CO METHANATION ; DEACTIVATION ; BIOMASS ; NICKEL ; SURFACE ; PHASE ; MODEL |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000317159300022 |
| 公开日期 | 2015-05-27 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/13595]  |
| 专题 | 过程工程研究所_研究所（批量导入） |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Jun,Zhou, Li,Li, Pengcheng,et al. Enhanced fluidized bed methanation over a Ni/Al2O3 catalyst for production of synthetic natural gas[J]. CHEMICAL ENGINEERING JOURNAL,2013,219(0):183-189. |
| APA | Li, Jun.,Zhou, Li.,Li, Pengcheng.,Zhu, Qingshan.,Gao, Jiajian.,...&Su, Fabing.(2013).Enhanced fluidized bed methanation over a Ni/Al2O3 catalyst for production of synthetic natural gas.CHEMICAL ENGINEERING JOURNAL,219(0),183-189. |
| MLA | Li, Jun,et al."Enhanced fluidized bed methanation over a Ni/Al2O3 catalyst for production of synthetic natural gas".CHEMICAL ENGINEERING JOURNAL 219.0(2013):183-189. |
入库方式： OAI收割
来源：过程工程研究所
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