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Photocatalytic Properties of Graphdiyne and Graphene Modified TiO2: From Theory to Experiment
文献类型：期刊论文
| 作者 | Yang, Nailiang1,5; Liu, Yuanyuan1; Wen, Hao1; Tang, Zhiyong2; Zhao, Huijun3; Li, Yuliang4; Wang, Dan1 |
| 刊名 | ACS NANO
 |
| 出版日期 | 2013-02-01 |
| 卷号 | 7期号:2页码:1504-1512 |
| 关键词 | graphdiyne graphene TiO2 composite crystal facet DFT calculation photocatalysis |
| 英文摘要 | The chemical structure and electronic properties of two-dimensional (2D) carbon-supported TiO2, TiO2-graphdiyne, and TiO2-graphene composites have been studied by first-principles density functional theory. Calculation results show that TiO2(001)-graphdiyne composites possess superior charge separation and oxidation properties, having the longest lifetimes of photoexcited carriers among all of the 2D composites containing TiO2 of different facets. Our experimental results further proved that TiO2(001)-graphdiyne composites could be a promising photocatalyst. For photocatalytic degradation of methylene blue, the rate constant of the TiO2(001)-graphdiyne composite is 1.63 +/- 0.15 times that of the pure TiO2(001) and 1.27 +/- 0.12 times that of the TiO2(001)-graphene composite. |
| WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
| 类目[WOS] | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
| 研究领域[WOS] | Chemistry ; Science & Technology - Other Topics ; Materials Science |
| 关键词[WOS] | VISIBLE-LIGHT IRRADIATION ; SENSITIZED SOLAR-CELLS ; TITANIUM-DIOXIDE ; 001 FACETS ; CARBON ; OXIDE ; HETEROJUNCTION ; NETWORKS ; SURFACE ; SHEETS |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000315618700071 |
| 公开日期 | 2015-05-27 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/13763]  |
| 专题 | 过程工程研究所_研究所（批量导入） |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 2.Natl Ctr Nanosci & Technol, Beijing, Peoples R China 3.Griffith Univ, Ctr Clean Environm & Energy, Griffith, Qld 4222, Australia 4.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Key Lab Organ Solids, Beijing 100190, Peoples R China 5.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Nailiang,Liu, Yuanyuan,Wen, Hao,et al. Photocatalytic Properties of Graphdiyne and Graphene Modified TiO2: From Theory to Experiment[J]. ACS NANO,2013,7(2):1504-1512. |
| APA | Yang, Nailiang.,Liu, Yuanyuan.,Wen, Hao.,Tang, Zhiyong.,Zhao, Huijun.,...&Wang, Dan.(2013).Photocatalytic Properties of Graphdiyne and Graphene Modified TiO2: From Theory to Experiment.ACS NANO,7(2),1504-1512. |
| MLA | Yang, Nailiang,et al."Photocatalytic Properties of Graphdiyne and Graphene Modified TiO2: From Theory to Experiment".ACS NANO 7.2(2013):1504-1512. |
入库方式： OAI收割
来源：过程工程研究所
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