Low-Temperature Reactivity of Zn+ Ions Confined in ZSM-5 Zeolite toward Carbon Monoxide Oxidation: Insight from in Situ DRIFT and ESR Spectroscopy
文献类型：期刊论文
| 作者 | Qi, Guodong1,2; Xu, Jun1,2; Su, Jihu3,4; Chen, Jiafu3,4; Wang, Xiumei1,2; Deng, Feng1,2 |
| 刊名 | JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
 |
| 出版日期 | 2013-05-08 |
| 卷号 | 135期号:18页码:6762-6765 |
| 英文摘要 | We report the low-temperature catalytic reactivity of Zn+ ions confined in ZSM-5 zeolite toward CO oxidation. In situ DRIFT and ESR spectroscopy demonstrated that molecular O-2 is readily activated by Zn+ ion to produce O-2(-) species at room temperature (298 K) via facile electron transfer between Zn+ ion and O-2 and that the formation of the active O-2(-) species is responsible for the high activity of the ZnZSM-5 catalyst toward CO oxidation. |
| WOS标题词 | Science & Technology ; Physical Sciences |
| 类目[WOS] | Chemistry, Multidisciplinary |
| 研究领域[WOS] | Chemistry |
| 关键词[WOS] | SOLID-STATE NMR ; CO OXIDATION ; CATALYTIC-OXIDATION ; PARAMAGNETIC RESONANCE ; ROOM-TEMPERATURE ; MFI ZEOLITE ; METHANE ; OXYGEN ; SURFACE ; AROMATIZATION |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000318839300006 |
| 公开日期 | 2015-07-14 |
| 源URL | [http://ir.wipm.ac.cn/handle/112942/955]  |
| 专题 | 武汉物理与数学研究所_磁共振应用研究部 |
| 作者单位 | 1.Chinese Acad Sci, Wuhan Ctr Magnet Resonance, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Peoples R China 2.Chinese Acad Sci, Wuhan Inst Phys & Math, Key Lab Magnet Resonance Biol Syst, Wuhan 430071, Peoples R China 3.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China 4.Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Peoples R China |
| 推荐引用方式 GB/T 7714 | Qi, Guodong,Xu, Jun,Su, Jihu,et al. Low-Temperature Reactivity of Zn+ Ions Confined in ZSM-5 Zeolite toward Carbon Monoxide Oxidation: Insight from in Situ DRIFT and ESR Spectroscopy[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2013,135(18):6762-6765. |
| APA | Qi, Guodong,Xu, Jun,Su, Jihu,Chen, Jiafu,Wang, Xiumei,&Deng, Feng.(2013).Low-Temperature Reactivity of Zn+ Ions Confined in ZSM-5 Zeolite toward Carbon Monoxide Oxidation: Insight from in Situ DRIFT and ESR Spectroscopy.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,135(18),6762-6765. |
| MLA | Qi, Guodong,et al."Low-Temperature Reactivity of Zn+ Ions Confined in ZSM-5 Zeolite toward Carbon Monoxide Oxidation: Insight from in Situ DRIFT and ESR Spectroscopy".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 135.18(2013):6762-6765. |
入库方式： OAI收割
来源：武汉物理与数学研究所
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