Micro/nano-structured graphitic carbon nitride-Ag nanoparticle hybrids as surface-enhanced Raman scattering substrates with much improved long-term stability
文献类型：期刊论文
| 作者 | Jiang, Jizhou1,2,3; Zhu, Lihua1; Zou, Jing4; Lei Ou-yang1,2,3; Zheng, Anmin5; Tang, Heqing2,3 |
| 刊名 | CARBON
 |
| 出版日期 | 2015-06-01 |
| 卷号 | 87页码:193-205 |
| 英文摘要 | Surface-enhanced Raman scattering (SERS) substrates with high SEAS activity and stability are important for SERS sensors. A facile method was developed to fabricate efficient and stable SERS substrates by combining Ag nanoparticles (NPs) and micro-scale sheeted graphitic carbon nitride (g-C3N4). The g-C3N4/Ag NPs hybrid could provide a great number of hot spots and concentrated the analyte by the pi-pi stacking interaction between analyte molecules and g-C3N4, making a dramatic Raman enhancement. Moreover, the g-C3N4/Ag NPs hybrid uniformly immobilized Ag NPs on the surface and edges of g-C3N4 sheets by an interaction between Ag NPs and g-C3N4, leading to much improved long-term stability. This could be explained in terms of the electron-donor effect of g-C3N4, which was further confirmed by density functional theory calculations. The inherent Raman enhancing effect of g-C3N4 itself also contributed to the total SERS responses. Due to multiple enhancement contributions, the g-C3N4/Ag NPs hybrid exhibited a strong Raman enhancement effect for with an enhancement factor of 4.6 x 10(8) (evaluated by using crystal violet as a probe), and possessed wide adaptability from dyes, pesticides to bio-molecules. (C) 2015 Elsevier Ltd. All rights reserved. |
| WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
| 类目[WOS] | Chemistry, Physical ; Materials Science, Multidisciplinary |
| 研究领域[WOS] | Chemistry ; Materials Science |
| 关键词[WOS] | REDUCED GRAPHENE OXIDE ; IN-SITU GROWTH ; PHOTOCATALYTIC ACTIVITY ; SILVER ELECTRODE ; COLLOIDAL SILVER ; SERS NANOTAGS ; LIVE CELLS ; SPECTROSCOPY ; CU2+ ; SPECTRA |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000352332900018 |
| 公开日期 | 2015-07-14 |
| 源URL | [http://ir.wipm.ac.cn/handle/112942/1068]  |
| 专题 | 武汉物理与数学研究所_磁共振应用研究部 |
| 作者单位 | 1.Huazhong Univ Sci & Technol, Coll Chem & Chem Engn, Wuhan 430074, Peoples R China 2.South Cent Univ Nationalities, Coll Chem & Mat Sci, Key Lab Catalysis & Mat Sci, State Ethn Affairs Commiss, Wuhan 430074, Peoples R China 3.South Cent Univ Nationalities, Coll Chem & Mat Sci, Minist Educ, Wuhan 430074, Peoples R China 4.Wuhan Inst Technol, Sch Chem & Environm Engn, Key Lab Green Chem Proc, Minist Educ, Wuhan 430073, Peoples R China 5.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Peoples R China |
| 推荐引用方式 GB/T 7714 | Jiang, Jizhou,Zhu, Lihua,Zou, Jing,et al. Micro/nano-structured graphitic carbon nitride-Ag nanoparticle hybrids as surface-enhanced Raman scattering substrates with much improved long-term stability[J]. CARBON,2015,87:193-205. |
| APA | Jiang, Jizhou,Zhu, Lihua,Zou, Jing,Lei Ou-yang,Zheng, Anmin,&Tang, Heqing.(2015).Micro/nano-structured graphitic carbon nitride-Ag nanoparticle hybrids as surface-enhanced Raman scattering substrates with much improved long-term stability.CARBON,87,193-205. |
| MLA | Jiang, Jizhou,et al."Micro/nano-structured graphitic carbon nitride-Ag nanoparticle hybrids as surface-enhanced Raman scattering substrates with much improved long-term stability".CARBON 87(2015):193-205. |
入库方式： OAI收割
来源：武汉物理与数学研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。