Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property
文献类型:期刊论文
作者 | Chen, Feitai1; Fang, Pengfei1; Liu, Zhi1; Gao, Yuanpeng1; Liu, Yang1; Dai, Yiqun1; Luo, Huan2; Feng, Jiwen2 |
刊名 | JOURNAL OF MATERIALS SCIENCE
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出版日期 | 2013-08-01 |
卷号 | 48期号:15页码:5171-5179 |
英文摘要 | TiO2-based nanostructures usually possess excellent photochemical properties. However, the relationship between their dimensionality and photocatalytic activity was rarely investigated. In this study, a series of TiO2-based nanostructures in various dimensionalities (such as nanosheets, nanotubes) were obtained by hydrothermal treatment of P25, and the process of structural evolution was also systematically investigated by TEM, BET, Raman, and XRD analysis. Much higher rate constant (3.7 x 10(-2) min(-1)) for the degradation of rhodamine B was found for nanosheets, comparing with those of three-dimensional P25 nanoparticles (0.59 x 10(-2) min(-1)) and one-dimensional nanotubes (0.85 x 10(-2) min(-1)). It is found that the hydrothermally prepared TiO2-based nanosheets possess small thickness (ca. 5 nm) and plentiful surface hydroxyl groups, and the reason why TiO2-based nanosheets possess superior photocatalytic activity is also discussed in detail from the microstructure and surface chemical states. In addition, TiO2-based nanosheets exhibit good reusability in the cyclic experiments, implying a potential application for photocatalytic degradation of organic pollutants. |
WOS标题词 | Science & Technology ; Technology |
类目[WOS] | Materials Science, Multidisciplinary |
研究领域[WOS] | Materials Science |
关键词[WOS] | TITANATE NANOTUBES ; FORMATION MECHANISM ; HYDROTHERMAL PROCESS ; TITANIUM-DIOXIDE ; TIO2 NANOTUBES ; 001 FACETS ; SPECTROSCOPY ; DEGRADATION ; PERFORMANCE ; COMPOSITES |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000319003300009 |
公开日期 | 2015-07-14 |
源URL | [http://ir.wipm.ac.cn/handle/112942/1538] ![]() |
专题 | 武汉物理与数学研究所_磁共振应用研究部 |
作者单位 | 1.Wuhan Univ, Key Lab Artificial Micro & Nanostruct, Minist Educ, Sch Phys & Technol, Wuhan 430072, Peoples R China 2.Chinese Acad Sci, Wuhan Inst Phys & Math, Wuhan 430071, Peoples R China |
推荐引用方式 GB/T 7714 | Chen, Feitai,Fang, Pengfei,Liu, Zhi,et al. Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property[J]. JOURNAL OF MATERIALS SCIENCE,2013,48(15):5171-5179. |
APA | Chen, Feitai.,Fang, Pengfei.,Liu, Zhi.,Gao, Yuanpeng.,Liu, Yang.,...&Feng, Jiwen.(2013).Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property.JOURNAL OF MATERIALS SCIENCE,48(15),5171-5179. |
MLA | Chen, Feitai,et al."Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property".JOURNAL OF MATERIALS SCIENCE 48.15(2013):5171-5179. |
入库方式: OAI收割
来源:武汉物理与数学研究所
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