中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property

文献类型:期刊论文

作者Chen, Feitai1; Fang, Pengfei1; Liu, Zhi1; Gao, Yuanpeng1; Liu, Yang1; Dai, Yiqun1; Luo, Huan2; Feng, Jiwen2
刊名JOURNAL OF MATERIALS SCIENCE
出版日期2013-08-01
卷号48期号:15页码:5171-5179
英文摘要TiO2-based nanostructures usually possess excellent photochemical properties. However, the relationship between their dimensionality and photocatalytic activity was rarely investigated. In this study, a series of TiO2-based nanostructures in various dimensionalities (such as nanosheets, nanotubes) were obtained by hydrothermal treatment of P25, and the process of structural evolution was also systematically investigated by TEM, BET, Raman, and XRD analysis. Much higher rate constant (3.7 x 10(-2) min(-1)) for the degradation of rhodamine B was found for nanosheets, comparing with those of three-dimensional P25 nanoparticles (0.59 x 10(-2) min(-1)) and one-dimensional nanotubes (0.85 x 10(-2) min(-1)). It is found that the hydrothermally prepared TiO2-based nanosheets possess small thickness (ca. 5 nm) and plentiful surface hydroxyl groups, and the reason why TiO2-based nanosheets possess superior photocatalytic activity is also discussed in detail from the microstructure and surface chemical states. In addition, TiO2-based nanosheets exhibit good reusability in the cyclic experiments, implying a potential application for photocatalytic degradation of organic pollutants.
WOS标题词Science & Technology ; Technology
类目[WOS]Materials Science, Multidisciplinary
研究领域[WOS]Materials Science
关键词[WOS]TITANATE NANOTUBES ; FORMATION MECHANISM ; HYDROTHERMAL PROCESS ; TITANIUM-DIOXIDE ; TIO2 NANOTUBES ; 001 FACETS ; SPECTROSCOPY ; DEGRADATION ; PERFORMANCE ; COMPOSITES
收录类别SCI
语种英语
WOS记录号WOS:000319003300009
公开日期2015-07-14
源URL[http://ir.wipm.ac.cn/handle/112942/1538]  
专题武汉物理与数学研究所_磁共振应用研究部
作者单位1.Wuhan Univ, Key Lab Artificial Micro & Nanostruct, Minist Educ, Sch Phys & Technol, Wuhan 430072, Peoples R China
2.Chinese Acad Sci, Wuhan Inst Phys & Math, Wuhan 430071, Peoples R China
推荐引用方式
GB/T 7714
Chen, Feitai,Fang, Pengfei,Liu, Zhi,et al. Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property[J]. JOURNAL OF MATERIALS SCIENCE,2013,48(15):5171-5179.
APA Chen, Feitai.,Fang, Pengfei.,Liu, Zhi.,Gao, Yuanpeng.,Liu, Yang.,...&Feng, Jiwen.(2013).Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property.JOURNAL OF MATERIALS SCIENCE,48(15),5171-5179.
MLA Chen, Feitai,et al."Dimensionality-dependent photocatalytic activity of TiO2-based nanostructures: nanosheets with a superior catalytic property".JOURNAL OF MATERIALS SCIENCE 48.15(2013):5171-5179.

入库方式: OAI收割

来源:武汉物理与数学研究所

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