中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Two-center interference in molecular photoelectron energy spectra with intense attosecond circularly polarized XUV laser pulses

文献类型:期刊论文

作者Yuan, Kai-Jun1; Bian, Xue-Bin2; Bandrauk, Andre D.1
刊名PHYSICAL REVIEW A
出版日期2014-08-06
卷号90期号:2
英文摘要We study two-center electron interference in molecular photoionization processes by intense attosecond circularly polarized extreme ultraviolet (XUV) laser pulses in both symmetric H-2(+) and nonsymmetric HHe2+ one-electron diatomic systems. Simulations from numerical solutions of time-dependent Schrodinger equations for the oriented symmetric molecular ion H-2(+) exhibit a signature of interference with double peaks (minima) in molecular attosecond photoelectron energy spectra (MAPES) at critical angles theta(c) between the continuum electron momentum p(e) and the molecular internuclear R axis. The interference patterns are shown to be influenced by the molecular Coulomb potential, leading to a shift of the critical angle theta(c). Dependence of the two-center interference on the pulse ellipticity is also investigated. Furthermore, it is found that the interference phenomena are critically sensitive to the molecular orbital symmetry. For the nonsymmetric molecular ion HHe2+, such double peaks in MAPES also occur, thus suggesting a method for imaging orbitals in molecules by intense ultrashort circularly polarized XUV pulses on the attosecond time scale.
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Optics ; Physics, Atomic, Molecular & Chemical
研究领域[WOS]Optics ; Physics
关键词[WOS]INDUCED ELECTRON-DIFFRACTION ; HARMONIC-GENERATION ; DIATOMIC-MOLECULES ; FIELD ; IONIZATION ; PHOTOIONIZATION ; EXCITATION ; DYNAMICS ; PHYSICS ; WAVE
收录类别SCI
语种英语
WOS记录号WOS:000341263600007
公开日期2015-07-14
源URL[http://ir.wipm.ac.cn/handle/112942/1429]  
专题武汉物理与数学研究所_理论与交叉研究部
作者单位1.Univ Sherbrooke, Fac Sci, Chim Theor Lab, Sherbrooke, PQ J1K 2R1, Canada
2.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Peoples R China
推荐引用方式
GB/T 7714
Yuan, Kai-Jun,Bian, Xue-Bin,Bandrauk, Andre D.. Two-center interference in molecular photoelectron energy spectra with intense attosecond circularly polarized XUV laser pulses[J]. PHYSICAL REVIEW A,2014,90(2).
APA Yuan, Kai-Jun,Bian, Xue-Bin,&Bandrauk, Andre D..(2014).Two-center interference in molecular photoelectron energy spectra with intense attosecond circularly polarized XUV laser pulses.PHYSICAL REVIEW A,90(2).
MLA Yuan, Kai-Jun,et al."Two-center interference in molecular photoelectron energy spectra with intense attosecond circularly polarized XUV laser pulses".PHYSICAL REVIEW A 90.2(2014).

入库方式: OAI收割

来源:武汉物理与数学研究所

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