Spatial distribution of perfluoroalkyl acids in surface sediments of the German Bight, North Sea
文献类型：期刊论文
| 作者 | Zhao, Zhen1,2,3; Xie, Zhiyong1; Tang, Jianhui3 ; Zhang, Gan2; Ebinghaus, Ralf1
|
| 刊名 | SCIENCE OF THE TOTAL ENVIRONMENT
 |
| 出版日期 | 2015-04-01 |
| 卷号 | 511页码:145-152 |
| 关键词 | Perfluoroalkyl acids Perfluorooctane sulfonic add Surface sediment German Bight |
| ISSN号 | 0048-9697 |
| 产权排序 | [Zhao, Zhen; Xie, Zhiyong; Ebinghaus, Ralf] Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, D-21502 Geesthacht, Germany; [Zhao, Zhen; Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510631, Guangdong, Peoples R China; [Zhao, Zhen; Tang, Jianhui] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China |
| 通讯作者 | Xie, ZY (reprint author), Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Max Plank St 1, D-21502 Geesthacht, Germany. zhiyong.xie@hzg.de ; jhtang@yic.ac.cn |
| 中文摘要 | Perfluoroalkyl adds (PFAAs) have been determined in the environment globally. However, studies on the occurrence of PFAAs in marine sediment remain limited. In this study, 16 PFAAs are investigated in surface sediments from the German Bight, which provided a good overview of the spatial distribution. The concentrations of Sigma PFAAs ranged from 0.056 to 7.4 ng/g dry weight. The highest concentration was found at the estuary of the River Ems, which might be the result of local discharge source. Perfluorooctane sulfonic acid (PFOS) was the dominant compound, and the enrichment of PFOS in sediment might be strongly related to the compound structure itself. The geographical condition of the German Bight influenced the movement of water and sediment, resulting in complex distribution. Following normalization according to total organic carbon (TOC) content, PFAA distributions showed a different picture. Significant linear relationships were found between total PFAA concentrations and TOC (R-2 = 0.50, p < 0.01). Compared with a previous study conducted in the same area, a declining trend was presented for the concentrations of PFOS and perfluorooctanoic acid (PFOA). Compound structure, geographical condition, and organic carbon in the sediment influence the distribution of PFAAs in the German Bight. Environmental risk assessment indicated that the risk from PFOA is negligible, whereas PFOS in marine sediment may present a risk for benthic organisms in the German Bight. (C) 2014 Elsevier B.V. All rights reserved. |
| 英文摘要 | Perfluoroalkyl adds (PFAAs) have been determined in the environment globally. However, studies on the occurrence of PFAAs in marine sediment remain limited. In this study, 16 PFAAs are investigated in surface sediments from the German Bight, which provided a good overview of the spatial distribution. The concentrations of Sigma PFAAs ranged from 0.056 to 7.4 ng/g dry weight. The highest concentration was found at the estuary of the River Ems, which might be the result of local discharge source. Perfluorooctane sulfonic acid (PFOS) was the dominant compound, and the enrichment of PFOS in sediment might be strongly related to the compound structure itself. The geographical condition of the German Bight influenced the movement of water and sediment, resulting in complex distribution. Following normalization according to total organic carbon (TOC) content, PFAA distributions showed a different picture. Significant linear relationships were found between total PFAA concentrations and TOC (R-2 = 0.50, p < 0.01). Compared with a previous study conducted in the same area, a declining trend was presented for the concentrations of PFOS and perfluorooctanoic acid (PFOA). Compound structure, geographical condition, and organic carbon in the sediment influence the distribution of PFAAs in the German Bight. Environmental risk assessment indicated that the risk from PFOA is negligible, whereas PFOS in marine sediment may present a risk for benthic organisms in the German Bight. (C) 2014 Elsevier B.V. All rights reserved. |
| 学科主题 | Environmental Sciences |
| 研究领域[WOS] | Environmental Sciences & Ecology |
| 关键词[WOS] | PERFLUORINATED ALKYL SUBSTANCES ; PERFLUOROOCTANE SULFONATE ; POLYFLUOROALKYL SUBSTANCES ; POLYFLUORINATED COMPOUNDS ; GLOBAL DISTRIBUTION ; YANGTZE-RIVER ; COASTAL AREAS ; WATER ; CHINA ; ATMOSPHERE |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000350513900016 |
| 源URL | [http://ir.yic.ac.cn/handle/133337/8638]  |
| 专题 | 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, D-21502 Geesthacht, Germany 2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510631, Guangdong, Peoples R China 3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Zhen,Xie, Zhiyong,Tang, Jianhui,et al. Spatial distribution of perfluoroalkyl acids in surface sediments of the German Bight, North Sea[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2015,511:145-152. |
| APA | Zhao, Zhen,Xie, Zhiyong,Tang, Jianhui,Zhang, Gan,&Ebinghaus, Ralf.(2015).Spatial distribution of perfluoroalkyl acids in surface sediments of the German Bight, North Sea.SCIENCE OF THE TOTAL ENVIRONMENT,511,145-152. |
| MLA | Zhao, Zhen,et al."Spatial distribution of perfluoroalkyl acids in surface sediments of the German Bight, North Sea".SCIENCE OF THE TOTAL ENVIRONMENT 511(2015):145-152. |
入库方式： OAI收割
来源：烟台海岸带研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。