中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Nanoreactor-confined synthesis and separation of yellow-luminescent graphene quantum dots with a recyclable SBA-15 template and their application for Fe(III) sensing

文献类型:期刊论文

作者Xu, HB (Xu, Hongbo); Zhou, SH (Zhou, Shenghai); Xiao, LL (Xiao, Lili); Li, SZ (Li, Shouzhu); Song, T (Song, Ting); Wang, Y (Wang, Yi); Yuan, QH (Yuan, Qunhui)
刊名CARBON
出版日期2015
卷号87期号:6页码:215-225
ISSN号0008-6223
英文摘要Graphene quantum dots (GQDs) have inspired growing research efforts. Although continuous progresses have been achieved in the syntheses of diverse GQDs, it is still a challenge in size-controllable and high-yield preparation of well dispersed GQDs via simple routes. Herein, we present a top-down synthesis of GQDs by using a SBA-15 template as a nanoreactor via a HNO3 vapor cutting strategy. With the recyclable ordered mesoporous SBA-15 template and a silica grid, a high-yield (48%) preparation as well as a facile separation of yellow-luminescent GQDs have been achieved. The obtained GQDs containing abundant oxygen-containing groups (ca. 30% for oxygen content) showed a narrow size distribution (2.5-5.2 nm), good water solubility, good photostability and high selectivity for Fe(III) sensing in tap water with satisfying recovery. Further experiments indicated that Cu(II), Co(II), Mn(II), Ni(II) could also quench the fluorescence of the as-prepared GQD after its surface states being adjusted, which might presage more possible applications of this material.
收录类别SCI
WOS记录号WOS:000352332900020
公开日期2015-07-11
源URL[http://ir.xjipc.cas.cn/handle/365002/4297]  
专题新疆理化技术研究所_环境科学与技术研究室
作者单位Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Lab Environm Sci & Technol, Key Lab Funct Mat & Devices Special Environm, Urumqi 830011, Peoples R China;Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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Xu, HB ,Zhou, SH ,Xiao, LL ,et al. Nanoreactor-confined synthesis and separation of yellow-luminescent graphene quantum dots with a recyclable SBA-15 template and their application for Fe(III) sensing[J]. CARBON,2015,87(6):215-225.
APA Xu, HB .,Zhou, SH .,Xiao, LL .,Li, SZ .,Song, T .,...&Yuan, QH .(2015).Nanoreactor-confined synthesis and separation of yellow-luminescent graphene quantum dots with a recyclable SBA-15 template and their application for Fe(III) sensing.CARBON,87(6),215-225.
MLA Xu, HB ,et al."Nanoreactor-confined synthesis and separation of yellow-luminescent graphene quantum dots with a recyclable SBA-15 template and their application for Fe(III) sensing".CARBON 87.6(2015):215-225.

入库方式: OAI收割

来源:新疆理化技术研究所

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