Direct synthesis of lanthanide-containing SBA-15 under weak acidic conditions and its catalytic study
文献类型:期刊论文
作者 | Mu, Zhen ; Li, Jin Jun ; Hao, Zheng Ping ; Qiao, Shi Zhang |
刊名 | MICROPOROUS AND MESOPOROUS MATERIALS
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出版日期 | 2008-08-01 |
卷号 | 113期号:2015-01-03页码:72-80 |
关键词 | weak acidic conditions mesoporous materials rare earth VOCs catalytic oxidation |
英文摘要 | Lanthanide (Ln including La, Cc and Nd) containing SBA-15 molecular sieves with molar ratio Ln/Si = 0.01-0.2 were prepared via direct synthesis under weak acidic conditions (pH 1.5-3.0). Characterizations of these samples were done by powder X-ray diffraction, N-2 adsorption, inductively coupled plasma atomic emission spectrometry (ICP-AES), FT-IR spectroscopy, and diffuse reflectance ultraviolet spectroscopy. All the samples show a highly ordered two-dimensional hexagonal mesostructure. N-2 adsorption testifies that all the Ln-containing SBA-15 materials have the type IV isotherms with type H-1 hysteresis loop as well as high specific surface area (798925 m(2)/g) and narrow pore size distribution. The diffuse reflectance UV-vis, ICP-AES, and the wide-angle XRD spectra show that most of the lanthanide ions are better dispersed in the calcined materials. The Ln-SBA-15 supported Pd catalysts show high catalytic activity in the oxidation of benzene. The results reveal that Ln-SBA-15 materials can be used as potential supports for the catalytic oxidation of Vocs. (C) 2007 Elsevier Inc. All rights reserved. |
WOS记录号 | WOS:000257362100010 |
源URL | [http://ir.rcees.ac.cn/handle/311016/22025] ![]() |
专题 | 生态环境研究中心_环境纳米材料实验室 |
推荐引用方式 GB/T 7714 | Mu, Zhen,Li, Jin Jun,Hao, Zheng Ping,et al. Direct synthesis of lanthanide-containing SBA-15 under weak acidic conditions and its catalytic study[J]. MICROPOROUS AND MESOPOROUS MATERIALS,2008,113(2015-01-03):72-80. |
APA | Mu, Zhen,Li, Jin Jun,Hao, Zheng Ping,&Qiao, Shi Zhang.(2008).Direct synthesis of lanthanide-containing SBA-15 under weak acidic conditions and its catalytic study.MICROPOROUS AND MESOPOROUS MATERIALS,113(2015-01-03),72-80. |
MLA | Mu, Zhen,et al."Direct synthesis of lanthanide-containing SBA-15 under weak acidic conditions and its catalytic study".MICROPOROUS AND MESOPOROUS MATERIALS 113.2015-01-03(2008):72-80. |
入库方式: OAI收割
来源:生态环境研究中心
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