Ionic degradation inhibitors and kinetic models for CO2 capture with aqueous monoethanolamine
文献类型：期刊论文
| 作者 | Zhao, Zhijun1,2; Dong, Haifeng1; Huang, Ying1,2; Cao, Lingdi1,2; Gao, Jubao1; Zhang, Xiangping1; Zhang, Suojiang1 |
| 刊名 | INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL
 |
| 出版日期 | 2015-08-01 |
| 卷号 | 39期号:AUG页码:119-128 |
| 关键词 | Degradation inhibitors Monoethanolamine Ionic Kinetics CO2 capture Notations List of symbols |
| ISSN号 | 1750-5836 |
| 英文摘要 | The degradation of monoethanolamine (MEA) solution was to be around 10% of the total cost of carbon dioxide (CO2) capture, thus, it is critically important to develop high efficient inhibitors. In this study, two novel ionic degradation inhibitors, monoethanolamine tartrate (MTA) and mercaptoethylamine tartrate (HTA) were synthesized. The results indicated that the inhibitive extent is in the order: MTA > KNaC4H4O6 > HTA > Na2SO3. The degradation kinetics of MEA solution with MTA was studied under conditions typical of the CO2 absorption process considering key factors, such as degradation temperature and aqueous phase concentrations of MEA, O-2, SO2, CO2, MTA and Fe2+. The degradation rate increases with the increases of temperature and concentrations of MEA, O-2 and SO2, whereas decreases with increasing concentrations of CO2 and ionic degradation inhibitor. The degradation kinetic model of MEA solution which firstly introduces the influences of the components of ionic degradation inhibitor and Fe2+ was proposed by fitting the experimental data. (C) 2015 Elsevier Ltd. All rights reserved. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Energy & Fuels ; Engineering, Environmental |
| 研究领域[WOS] | Energy & Fuels ; Engineering |
| 关键词[WOS] | FLUE-GAS STREAMS ; OXIDATIVE-DEGRADATION ; CARBON-DIOXIDE ; ABSORPTION ; PLANT ; MEA ; PRODUCTS ; LIQUIDS ; PATHWAYS ; PROGRESS |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000358627100011 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/19416]  |
| 专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Key Lab Green Proc & Engn,Inst Proc Engn, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Zhijun,Dong, Haifeng,Huang, Ying,et al. Ionic degradation inhibitors and kinetic models for CO2 capture with aqueous monoethanolamine[J]. INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL,2015,39(AUG):119-128. |
| APA | Zhao, Zhijun.,Dong, Haifeng.,Huang, Ying.,Cao, Lingdi.,Gao, Jubao.,...&Zhang, Suojiang.(2015).Ionic degradation inhibitors and kinetic models for CO2 capture with aqueous monoethanolamine.INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL,39(AUG),119-128. |
| MLA | Zhao, Zhijun,et al."Ionic degradation inhibitors and kinetic models for CO2 capture with aqueous monoethanolamine".INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL 39.AUG(2015):119-128. |
入库方式： OAI收割
来源：过程工程研究所
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