The oxidative coupling of methane and the aromatization of methane without using oxidants
文献类型:期刊论文
作者 | Xie, MS; Chen, WH; Wang, XL; Xu, GF; Yang, X; Tao, LX; Guo, XX; Parmaliana, A; Sanfilippo, D; Frusteri, F |
刊名 | natural gas conversion v
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出版日期 | 1998 |
卷号 | 119页码:319-324 |
关键词 | methane oxidative coupling aromatization benzene HZSM-5 |
英文摘要 | it is found that the water in cofeed gas had three kinds of effects on the oxidative coupling of methane: 1) decrease in the temperature of catalyst bed and increase in the selectivity of coupling products 2) a rise in the temperature of catalyst bed 3) oscillating in the temperature of catalyst bed. those mainly depend on the properties of the catalysts and operation conditions. mie have developed the radial now fixed bed reactor for the oxidative coupling of methane, which may maintain the good performance of catalysts an the larger test scale. it is proposed that the methane aromatization on the mo/zsm-5 zeolite catalyst without using oxidants is a structure sensitive reaction and the deactivation of the catalyst is initially related to the reduction of the mo species at higher valence and loss of surface oxygen. the equation of the coke forming is listed. |
WOS标题词 | science & technology ; physical sciences ; technology |
类目[WOS] | chemistry, applied ; chemistry, physical ; engineering, chemical |
研究领域[WOS] | chemistry ; engineering |
关键词[WOS] | location ; cations ; zsm-5 |
收录类别 | ISTP ; SCI |
语种 | 英语 |
WOS记录号 | WOS:000076939000051 |
公开日期 | 2015-11-10 |
源URL | [http://159.226.238.44/handle/321008/138201] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
作者单位 | Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China |
推荐引用方式 GB/T 7714 | Xie, MS,Chen, WH,Wang, XL,et al. The oxidative coupling of methane and the aromatization of methane without using oxidants[J]. natural gas conversion v,1998,119:319-324. |
APA | Xie, MS.,Chen, WH.,Wang, XL.,Xu, GF.,Yang, X.,...&Arena, F.(1998).The oxidative coupling of methane and the aromatization of methane without using oxidants.natural gas conversion v,119,319-324. |
MLA | Xie, MS,et al."The oxidative coupling of methane and the aromatization of methane without using oxidants".natural gas conversion v 119(1998):319-324. |
入库方式: OAI收割
来源:大连化学物理研究所
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