中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Cluster-assisted multiple ionization of methyl iodide by a nanosecond laser: Influence of laser intensity on the kinetic energy and peak profile of multicharged ions

文献类型:期刊论文

作者Wen, LH; Li, HY; Luo, XL; Niu, DM; Xiao, X; Wang, B; Liang, F; Hou, KY; Shao, SY
刊名chemical physics
出版日期2006-03-20
卷号322期号:3页码:360-365
关键词methyl iodide multiple ionization cluster space charge effect
英文摘要the dependences of kinetic energies and peak profiles of multicharged ions of iq+ (q = 2-3) and c2+ on the laser intensity have been studied in detail by time-of-flight mass spectrometry, those multicharged ions are produced by irradiation of methyl iodide cluster beam with a nanosecond 532 nm nd-yag laser. our experiments show that the kinetic energies released of multicharged ions increase linearly with the laser intensity in the range of 3 x 10(9)-2 x 10(11) w/cm(2). the peaks of multicharged ions are split to forward ions and backward ions, and the ratio of the backward ions to forward ions decreases exponentially with laser intensity. the decreasing of backward ions is probably due to coulomb scattering by the heavier i+ ions when they turn around through the laser focus point. the linear dependence of kinetic energy of multicharged ions on laser intensity is interpreted by the ionization mechanism, in which the laser induced inverse bremsstrahlung heating of electron is the rate-limiting step. (c) 2005 elsevier b.v. all rights reserved.
WOS标题词science & technology ; physical sciences
类目[WOS]chemistry, physical ; physics, atomic, molecular & chemical
研究领域[WOS]chemistry ; physics
关键词[WOS]x-ray-emission ; coulomb explosion ; multiphoton ionization ; molecular clusters ; electron dynamics ; nuclear-dynamics ; atomic clusters ; generation ; fields ; pulses
收录类别SCI
语种英语
WOS记录号WOS:000236318200014
公开日期2015-11-17
源URL[http://159.226.238.44/handle/321008/140264]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Opt & Techol, Hefei 230031, Peoples R China
推荐引用方式
GB/T 7714
Wen, LH,Li, HY,Luo, XL,et al. Cluster-assisted multiple ionization of methyl iodide by a nanosecond laser: Influence of laser intensity on the kinetic energy and peak profile of multicharged ions[J]. chemical physics,2006,322(3):360-365.
APA Wen, LH.,Li, HY.,Luo, XL.,Niu, DM.,Xiao, X.,...&Shao, SY.(2006).Cluster-assisted multiple ionization of methyl iodide by a nanosecond laser: Influence of laser intensity on the kinetic energy and peak profile of multicharged ions.chemical physics,322(3),360-365.
MLA Wen, LH,et al."Cluster-assisted multiple ionization of methyl iodide by a nanosecond laser: Influence of laser intensity on the kinetic energy and peak profile of multicharged ions".chemical physics 322.3(2006):360-365.

入库方式: OAI收割

来源:大连化学物理研究所

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