Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces
文献类型：期刊论文
| 作者 | Zhang, Wen-kai; Wang, Hong-fei; Zheng, De-sheng |
| 刊名 | physical chemistry chemical physics
 |
| 出版日期 | 2006 |
| 卷号 | 8期号:35页码:4041-4052 |
| 英文摘要 | second harmonic generation (shg) has been proven a uniquely effective technique in the investigation of molecular structure and conformations, as well as dynamics of molecular interfaces. the ability to apply shg to molecular interface studies depends on the ability to abstract quantitative information from the measurable quantities in the actual shg experiments. in this review, we try to assess recent developments in the shg experimental methodologies towards quantitative analysis of the nonlinear optical properties of the achiral molecular interfaces with rotational isotropy along the interface normal. these developments include the methodology for orientational analysis of the shg experimental data, the experimental approaches for more accurate shg measurements, and a novel treatment of the symmetry properties of the molecular polarizability tensors in association with the experimentally measurable quantities. in the end, the recent developments on the problem of surface versus bulk contribution in shg surface studies is discussed. these developments can put shg on a more solid foundation for molecular interface studies, and to pave the way for better understanding and application of shg surface studies in general. |
| WOS标题词 | science & technology ; physical sciences |
| 类目[WOS] | chemistry, physical ; physics, atomic, molecular & chemical |
| 研究领域[WOS] | chemistry ; physics |
| 关键词[WOS] | 2nd harmonic-generation ; sum-frequency generation ; orientation-insensitive methodology ; surface vibrational spectroscopy ; self-assembled monolayers ; langmuir-blodgett-films ; air-water-interface ; multipolar contributions ; air/water interface ; isotropic fluids |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000240109300001 |
| 公开日期 | 2015-11-17 |
| 源URL | [http://159.226.238.44/handle/321008/140330]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, State Key Lab Mol React Dynam, Beijing 100080, Peoples R China 2.Grad Univ Chinese Acad Sci, Beijing 100864, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Wen-kai,Wang, Hong-fei,Zheng, De-sheng. Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces[J]. physical chemistry chemical physics,2006,8(35):4041-4052. |
| APA | Zhang, Wen-kai,Wang, Hong-fei,&Zheng, De-sheng.(2006).Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces.physical chemistry chemical physics,8(35),4041-4052. |
| MLA | Zhang, Wen-kai,et al."Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces".physical chemistry chemical physics 8.35(2006):4041-4052. |
入库方式： OAI收割
来源：大连化学物理研究所
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