Three-state model for femtosecond broadband stimulated Raman scattering
文献类型：期刊论文
| 作者 | Sun, Z.1; Qiu, Xue Q.1; Lu, J.2; Zhang, Dong H.3,4; Lee, Soo-Y.1 |
| 刊名 | journal of raman spectroscopy
 |
| 出版日期 | 2008-11-01 |
| 卷号 | 39期号:11页码:1568-1577 |
| 关键词 | femtosecond stimulated Raman scattering inverse Raman scattering nonlinear processes |
| 英文摘要 | stimulated raman scattering (srs) is analyzed with a three-state model. using a diagrammatic density-matrix formalism, srs by a pair of raman pump and probe pulses, with observation along the probe direction, is described principally by eight terms. the eight terms can be grouped into four sets, which are labeled as srs or irs (inverse raman scattering): srs(i), srs(id, irs(i), and irs(ii). specializing to the case of femtosecond srs (fsrs) by a picosecond (ps) raman pump pulse and a femtosecond (fs) probe pulse, the spectra for the four sets of terms under off-resonance and resonance conditions were calculated. the results obtained can explain the fsrs experimental observations from a (decaying) stationary vibrational state, such as (1) high wavenumber resolution (determined by the narrow bandwidth raman pump pulse) and high time resolution (deter-mined by the fs probe pulse), (2) stokes gain vs anti-stokes loss in off-resonance fsrs, and (3) dispersive lineshapes in resonance fsrs. copyright (c) 2008 john wiley & sons, ltd. |
| WOS标题词 | science & technology ; technology |
| 类目[WOS] | spectroscopy |
| 研究领域[WOS] | spectroscopy |
| 关键词[WOS] | excited-state ; beta-carotene ; ultrafast dynamics ; spectroscopy |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000261206200010 |
| 公开日期 | 2015-11-17 |
| 源URL | [http://159.226.238.44/handle/321008/141052]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637616, Singapore 2.Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China 3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 4.Chinese Acad Sci, Dalian Inst Chem Phys, Ctr Theoret & Computat Chem, Dalian 116023, Peoples R China |
| 推荐引用方式 GB/T 7714 | Sun, Z.,Qiu, Xue Q.,Lu, J.,et al. Three-state model for femtosecond broadband stimulated Raman scattering[J]. journal of raman spectroscopy,2008,39(11):1568-1577. |
| APA | Sun, Z.,Qiu, Xue Q.,Lu, J.,Zhang, Dong H.,&Lee, Soo-Y..(2008).Three-state model for femtosecond broadband stimulated Raman scattering.journal of raman spectroscopy,39(11),1568-1577. |
| MLA | Sun, Z.,et al."Three-state model for femtosecond broadband stimulated Raman scattering".journal of raman spectroscopy 39.11(2008):1568-1577. |
入库方式： OAI收割
来源：大连化学物理研究所
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