Mass transfer characteristics of H2S absorption from gaseous mixture into methyldiethanolamine solution in a T-junction microchannel
文献类型：期刊论文
| 作者 | Su, Hongjiu1,2; Wang, Shudong1; Niu, Haining1; Pan, Liwei1; Wang, Anjie2; Hu, Yongkang2 |
| 刊名 | separation and purification technology
 |
| 出版日期 | 2010-05-11 |
| 卷号 | 72期号:3页码:326-334 |
| 关键词 | Absorption Microreactor Mass transfer Process intensification Interfacial area |
| 英文摘要 | in this work, the mass transfer characteristics of absorption of h2s (1200 ppmv) into 40 wt% methyldiethanolamine (mdea) solution have been investigated experimentally in a horizontal cross-flow t-junction microchannel with a diameter of 1.00 mm. the interfacial area was determined by the absorption of co2 into naoh solution. it was found that the high removal efficiency of h2s (up to 99.5%) was achieved in the microchannel. mass transfer resistance existed mainly on the gas side in this absorption process. it was shown that the gas side volumetric mass transfer coefficient and interfacial area were as high as 31,746 mol/(m(3) s atm) and 11,100 m(2)/m(3), respectively. in addition, a comparison of mass transfer performance among different gas-liquid contactors was performed. it was revealed that the t-junction microchannel in this study could provide at least one or two orders of magnitude higher gas side volumetric mass transfer coefficient than others. however, the intensification of mass transfer process was mainly ascribed to the enhancement of interfacial area rather than the gas side mass transfer coefficient. empirical correlations based on the experimental data were developed to predict gas side mass transfer coefficient and interfacial area. published by elsevier b.v. |
| WOS标题词 | science & technology ; technology |
| 类目[WOS] | engineering, chemical |
| 研究领域[WOS] | engineering |
| 关键词[WOS] | cocurrent 2-phase flow ; aqueous blended amines ; gas-liquid flow ; structured packing ; hydrogen-sulfide ; carbon-dioxide ; selective absorption ; capillaries ; solubility ; bubbles |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000277662200014 |
| 公开日期 | 2015-11-17 |
| 源URL | [http://159.226.238.44/handle/321008/142181]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 2.Dalian Univ Technol, State Key Lab Fine Chem, Dalian 116012, Peoples R China |
| 推荐引用方式 GB/T 7714 | Su, Hongjiu,Wang, Shudong,Niu, Haining,et al. Mass transfer characteristics of H2S absorption from gaseous mixture into methyldiethanolamine solution in a T-junction microchannel[J]. separation and purification technology,2010,72(3):326-334. |
| APA | Su, Hongjiu,Wang, Shudong,Niu, Haining,Pan, Liwei,Wang, Anjie,&Hu, Yongkang.(2010).Mass transfer characteristics of H2S absorption from gaseous mixture into methyldiethanolamine solution in a T-junction microchannel.separation and purification technology,72(3),326-334. |
| MLA | Su, Hongjiu,et al."Mass transfer characteristics of H2S absorption from gaseous mixture into methyldiethanolamine solution in a T-junction microchannel".separation and purification technology 72.3(2010):326-334. |
入库方式： OAI收割
来源：大连化学物理研究所
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