中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Theoretical study of the photodissociation of Li-2(+) in one-color intense laser fields

文献类型:期刊论文

作者Li, Yuanjun1,2; Jiang, Wanyi3; Khait, Yuriy G.3; Hoffmann, Mark R.3
刊名journal of chemical physics
出版日期2011-05-07
卷号134期号:17
英文摘要a theoretical treatment of the photodissociation of the molecular ion li-2(+) in one-color intense laser fields, using the time-dependent wave packet approach in a floquet born-oppenheimer representation, is presented. six electronic states 1,2(2)sigma(g)+, 1,2(2)sigma(u)+, 1 (2)pi(g), and 1 (2)pi(u) are of relevance in this simulation and have been included. the dependences of the fragmental dissociation probabilities and kinetic energy release (ker) spectra on pulse width, peak intensity, polarization angle, wavelength, and initial vibrational level are analyzed to interpret the influence of control parameters of the external field. three main dissociation channels, 1 (2)sigma(g)+ (m = -1), 2 (2)sigma(g)+ (m = -2), and 2 (2)sigma(u)+ (m = -3), are seen to dominate the dissociation processes under a wide variety of laser conditions and give rise to well separated groups of ker features. different dissociation mechanisms for the involved floquet channels are discussed. (c) 2011 american institute of physics. [doi:10.1063/1.3585645]
WOS标题词science & technology ; physical sciences
类目[WOS]physics, atomic, molecular & chemical
研究领域[WOS]physics
关键词[WOS]above-threshold-dissociation ; quantum-mechanical system ; dependent wave-packet ; floquet states ; schrodinger-equation ; wavepacket dynamics ; rabi oscillations ; coherent control ; rydberg states ; ground-state
收录类别SCI
语种英语
WOS记录号WOS:000290393200014
公开日期2015-11-17
源URL[http://159.226.238.44/handle/321008/142444]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
3.Univ N Dakota, Dept Chem, Grand Forks, ND 58202 USA
推荐引用方式
GB/T 7714
Li, Yuanjun,Jiang, Wanyi,Khait, Yuriy G.,et al. Theoretical study of the photodissociation of Li-2(+) in one-color intense laser fields[J]. journal of chemical physics,2011,134(17).
APA Li, Yuanjun,Jiang, Wanyi,Khait, Yuriy G.,&Hoffmann, Mark R..(2011).Theoretical study of the photodissociation of Li-2(+) in one-color intense laser fields.journal of chemical physics,134(17).
MLA Li, Yuanjun,et al."Theoretical study of the photodissociation of Li-2(+) in one-color intense laser fields".journal of chemical physics 134.17(2011).

入库方式: OAI收割

来源:大连化学物理研究所

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