Real-time visualization of the dynamic evolution of CS2 4d and 6s Rydberg wave packet components
文献类型：期刊论文
| 作者 | Long, Jinyou1,2; Liu, Yuzhu1,2; Qin, Chaochao1,2; Zhang, Song1,2; Zhang, Bing1,2 |
| 刊名 | OPTICS EXPRESS
 |
| 出版日期 | 2011-02-28 |
| 卷号 | 19期号:5页码:4542-4552 |
| 英文摘要 | The dynamic evolution of CS2 4d and 6s Rydberg wave packet components has been experimentally visualized via femtosecond time-resolved photoelectron imaging coupled with time-resolved mass spectroscopy. The temporal evolution of the four components of the prepared Rydberg wave packet is directly observed as time-dependent changes of the intensities of different parts in the main photoelectron peak. Furthermore, time-resolved photoelectron angular distributions (PADs) clearly reflect the different component characters of 4d and 6s molecular orbitals. The lifetime of Rydberg wave packets is determined to be about 830fs and their decay is attributed to predissociation. Our results suggest the possibility of directly visualizing and determining the amplitudes and relative phases of different electronic and vibrational wave packet components in polyatomic molecules. (C) 2011 Optical Society of America |
| WOS标题词 | Science & Technology ; Physical Sciences |
| 类目[WOS] | Optics |
| 研究领域[WOS] | Optics |
| 关键词[WOS] | RESOLVED PHOTOELECTRON-SPECTROSCOPY ; (1+1)+1 MULTIPHOTON IONIZATION ; KINETIC-ENERGY PHOTOELECTRON ; SUB-DOPPLER SPECTROSCOPY ; FEMTOSECOND PUMP-PROBE ; FRACTIONAL REVIVALS ; ULTRAFAST DYNAMICS ; LARGE MOLECULES ; STATE ; CLUSTERS |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000288870300079 |
| 公开日期 | 2015-12-01 |
| 源URL | [http://ir.wipm.ac.cn/handle/112942/8225]  |
| 专题 | 武汉物理与数学研究所_2011年以前论文发表（包括2011年） |
| 作者单位 | 1.Chinese Acad Sci Wuhan, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Natl Lab Optoelect, Wuhan 430071, Hebei, Peoples R China 2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Long, Jinyou,Liu, Yuzhu,Qin, Chaochao,et al. Real-time visualization of the dynamic evolution of CS2 4d and 6s Rydberg wave packet components[J]. OPTICS EXPRESS,2011,19(5):4542-4552. |
| APA | Long, Jinyou,Liu, Yuzhu,Qin, Chaochao,Zhang, Song,&Zhang, Bing.(2011).Real-time visualization of the dynamic evolution of CS2 4d and 6s Rydberg wave packet components.OPTICS EXPRESS,19(5),4542-4552. |
| MLA | Long, Jinyou,et al."Real-time visualization of the dynamic evolution of CS2 4d and 6s Rydberg wave packet components".OPTICS EXPRESS 19.5(2011):4542-4552. |
入库方式： OAI收割
来源：武汉物理与数学研究所
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