A structured packed-bed reactor designed for exothermic hydrogenation of acetone
文献类型:期刊论文
作者 | Duan, Yanjun1,2; Xu, Min1; Zhou, Xiaoming1; Huai, Xiulan1 |
刊名 | PARTICUOLOGY
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出版日期 | 2014-12-01 |
卷号 | 17页码:125-130 |
关键词 | Chemical heat pump Structured packed-bed reactor Acetone hydrogenation CFD simulation |
英文摘要 | Fixed-bed reactors randomly packed with catalysts have many disadvantages that may adversely affect the desired chemical reaction. The increasingly used monolithic reactor, in contrast, has many operational advantages; however, for a kinetically-controlled reaction, it does not contain sufficient catalyst to sustain the reaction. To address the problems associated with both randomly packed-bed reactor and the monolithic reactor, a structured packed-bed reactor was proposed and mathematical models were built for randomly packed-bed reactor and structured packed-bed reactor. Their respective performances were compared when applied to the exothermic reaction of the isopropanol-acetone-hydrogen chemical heat pump system. The results showed that the structured packed-bed reactor performed better in terms of pressure drop and heat transfer capacity, and had a lower radial temperature gradient, indicating that this reactor had a higher effective heat conductivity. Isopropanol on the catalyst particle surfaces was more concentrated near the tube wall because a wall effect existed in the boundary layer around the particle-wall contact points. (C) 2013 Published by Elsevier B.V. on behalf of Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. |
WOS标题词 | Science & Technology ; Technology |
类目[WOS] | Engineering, Chemical ; Materials Science, Multidisciplinary |
研究领域[WOS] | Engineering ; Materials Science |
关键词[WOS] | CHEMICAL HEAT-PUMP |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000347656700018 |
公开日期 | 2015-12-22 |
源URL | [http://ir.etp.ac.cn/handle/311046/106074] ![]() |
专题 | 工程热物理研究所_中国科学院工程热物理所(论文库)_期刊论文(SCI) |
作者单位 | 1.Chinese Acad Sci, Inst Engn Thermophys, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Duan, Yanjun,Xu, Min,Zhou, Xiaoming,et al. A structured packed-bed reactor designed for exothermic hydrogenation of acetone[J]. PARTICUOLOGY,2014,17:125-130. |
APA | Duan, Yanjun,Xu, Min,Zhou, Xiaoming,&Huai, Xiulan.(2014).A structured packed-bed reactor designed for exothermic hydrogenation of acetone.PARTICUOLOGY,17,125-130. |
MLA | Duan, Yanjun,et al."A structured packed-bed reactor designed for exothermic hydrogenation of acetone".PARTICUOLOGY 17(2014):125-130. |
入库方式: OAI收割
来源:工程热物理研究所
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