Experimental investigation of hydrogen production integrated methanol steam reforming with middle-temperature solar thermal energy
文献类型:期刊论文
作者 | Liu, Qibin1,2; Hong, Hui1; Yuan, Jianli1,2; Jin, Hongguang1; Cai, Ruixian1 |
刊名 | APPLIED ENERGY
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出版日期 | 2009-02-01 |
卷号 | 86期号:2页码:155-162 |
关键词 | Hydrogen production Methanol steam reforming Middle-temperature solar reactor Kinetic model |
英文摘要 | Developing a hydrogen production method that utilizes solar thermal energy in an effective manner is a great challenge. In this paper we propose a new approach to solar hydrogen production with the integration of methanol steam reforming and middle-temperature solar thermal energy. An experiment on hydrogen production is conducted using a 5-kW solar reactor at 150-300 degrees C under atmosphere pressure. The 5-kW solar receiver/reactor is fabricated and positioned along the focal line of one-tracking parabolic trough concentrator. As a result, the chemical conversion of methanol can reach levels higher than 90%, and the volumetric concentration of hydrogen in the gas products can account for 66-74% above the solar flux of 580 W/m(2). The obtained maximum hydrogen yield per mole of methanol is 2.65-2.90 mol, approaching the theoretical maximum value. and the experimentally obtained thermo-chemical efficiency of solar thermal energy converted into chemical energy is in the range of 30-50%, which is competitive with other high-temperature solar thermochemical processes. A kinetic model of solar-driven methanol steam reforming related to solar flux is also derived based on the experimental data. The promising results demonstrate that this solar-driven hydrogen production method can be feasible in practical applications. (c) 2008 Elsevier Ltd. All rights reserved. |
WOS标题词 | Science & Technology ; Technology |
类目[WOS] | Energy & Fuels ; Engineering, Chemical |
研究领域[WOS] | Energy & Fuels ; Engineering |
关键词[WOS] | CU/ZNO/AL2O3 CATALYST ; GASIFICATION ; KINETICS ; POWER |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000260269000005 |
公开日期 | 2015-12-22 |
源URL | [http://ir.etp.ac.cn/handle/311046/106388] ![]() |
专题 | 工程热物理研究所_中国科学院工程热物理所(论文库)_期刊论文(SCI) |
作者单位 | 1.Chinese Acad Sci, Inst Engn Thermophys, Beijing 100080, Peoples R China 2.Chinese Acad Sci, Grad Sch, Beijing 100080, Peoples R China |
推荐引用方式 GB/T 7714 | Liu, Qibin,Hong, Hui,Yuan, Jianli,et al. Experimental investigation of hydrogen production integrated methanol steam reforming with middle-temperature solar thermal energy[J]. APPLIED ENERGY,2009,86(2):155-162. |
APA | Liu, Qibin,Hong, Hui,Yuan, Jianli,Jin, Hongguang,&Cai, Ruixian.(2009).Experimental investigation of hydrogen production integrated methanol steam reforming with middle-temperature solar thermal energy.APPLIED ENERGY,86(2),155-162. |
MLA | Liu, Qibin,et al."Experimental investigation of hydrogen production integrated methanol steam reforming with middle-temperature solar thermal energy".APPLIED ENERGY 86.2(2009):155-162. |
入库方式: OAI收割
来源:工程热物理研究所
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