Highly efficient Z-Scheme Ag3PO4/Ag/WO3-x photocatalyst for its enhanced photocatalytic performance
文献类型:期刊论文
作者 | Bu, Yuyu1; Chen, Zhuoyuan1; Sun, Chengjun2 |
刊名 | APPLIED CATALYSIS B-ENVIRONMENTAL
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出版日期 | 2015-12-01 |
卷号 | 179期号:179页码:363-371 |
关键词 | Z-scheme WO2.72 Ag Ag3PO4/Ag/WO3-x |
英文摘要 | The Z-Scheme Ag3PO4/Ag/WO3-x photocatalyst was prepared through an in situ deposition method. Originally, WO2.72 with hierarchical sea urchin-like structure was mixed with excessive Ag+ ions. The weak reducibility of WO2.72 was utilized to in situ reduce Ag+ into Ag, and Ag nanoparticles were deposited on the surface of WO2.72. Subsequently, an appropriate amount of PO43- ions was directly added dropwise to combine with the remaining Ag+ ions, as a result, the Ag3PO4 nanoparticles was, therefore, in situ deposited on the surface of Ag/WO3-x, and the Z-Scheme Ag3PO4/Ag/WO3-x photocatalyst was obtained. The experimental results illustrate that, for the Z-Scheme Ag3PO4/Ag/WO3-x photocatalyst, Ag nanoparticles serve as carrier-transfer centers, effectively prolong the lifetime of the photoinduced electrons generated by Ag3PO4 and the photoinduced holes generated by WO3-x, and therefore improve the photocatalytic degradation performance. The utilization of the weak reducibility of the transition metal oxides has been explored as an effective strategy to fabricate Z-scheme 'reduced state transition metal oxide/noble metal/semiconductor' photocatalysts with enhanced photocatalytic performance. (C) 2015 Elsevier B.V. All rights reserved. |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000359873800040 |
源URL | [http://ir.qdio.ac.cn/handle/337002/50102] ![]() |
专题 | 海洋研究所_海洋腐蚀与防护研究发展中心 |
作者单位 | 1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China 2.State Ocean Adm, Inst Oceanog 1, Marine Ecol Ctr, Qingdao 266061, Peoples R China |
推荐引用方式 GB/T 7714 | Bu, Yuyu,Chen, Zhuoyuan,Sun, Chengjun. Highly efficient Z-Scheme Ag3PO4/Ag/WO3-x photocatalyst for its enhanced photocatalytic performance[J]. APPLIED CATALYSIS B-ENVIRONMENTAL,2015,179(179):363-371. |
APA | Bu, Yuyu,Chen, Zhuoyuan,&Sun, Chengjun.(2015).Highly efficient Z-Scheme Ag3PO4/Ag/WO3-x photocatalyst for its enhanced photocatalytic performance.APPLIED CATALYSIS B-ENVIRONMENTAL,179(179),363-371. |
MLA | Bu, Yuyu,et al."Highly efficient Z-Scheme Ag3PO4/Ag/WO3-x photocatalyst for its enhanced photocatalytic performance".APPLIED CATALYSIS B-ENVIRONMENTAL 179.179(2015):363-371. |
入库方式: OAI收割
来源:海洋研究所
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