Experimental study of enhanced phosphogypsum carbonation with ammonia under increased CO2 pressure
文献类型：期刊论文
| 作者 | Zhao, Hongtao1,2; Li, Huiquan1; Bao, Weijun1; Wang, Chenye1; Li, Songgeng2; Lin, Weigang2 |
| 刊名 | JOURNAL OF CO2 UTILIZATION
 |
| 出版日期 | 2015-09-01 |
| 卷号 | 11期号:SEP页码:10-19 |
| 关键词 | Calcite Phosphogypsum Ammonium Accelerated carbonation Increased CO2 pressure |
| ISSN号 | 2212-9820 |
| 英文摘要 | Phosphogypsum is the byproduct discharged from phosphate industry. A novel process was proposed for converting phosphogypsum into ammonium sulfate via phosphogypsum carbonation with ammonia. The effects of stirring speed, reaction time, initial temperature, CO2 partial pressure, liquid-solid ratio and excess ammonia ratio were evaluated. The main phases presented before and after the carbonation process were identified using X-ray fluorescence (XRF), X-ray diffraction (XRD), scanning electron microscopy with energy dispersive X-ray (SEM-EDX) and carbon-sulfur (CS) analytical techniques. The phosphogypsum was found to have the highest carbonation conversion of approximately 97% in 5 min. The product collected from the reaction was characterized as calcite with the average particle size smaller than the raw phosphogypsum. (C) 2014 Elsevier Ltd. All rights reserved. |
| WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
| 类目[WOS] | Chemistry, Multidisciplinary ; Engineering, Chemical |
| 研究领域[WOS] | Chemistry ; Engineering |
| 关键词[WOS] | GAS DESULFURIZATION GYPSUM ; MINERAL CARBONATION ; AQUEOUS CARBONATION ; SEQUESTRATION ; PARAMETERS ; PRODUCTS ; WASTE |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000361861600003 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/19580]  |
| 专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Clean Prod Technol Hydromet, Beijing 100080, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100080, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Hongtao,Li, Huiquan,Bao, Weijun,et al. Experimental study of enhanced phosphogypsum carbonation with ammonia under increased CO2 pressure[J]. JOURNAL OF CO2 UTILIZATION,2015,11(SEP):10-19. |
| APA | Zhao, Hongtao,Li, Huiquan,Bao, Weijun,Wang, Chenye,Li, Songgeng,&Lin, Weigang.(2015).Experimental study of enhanced phosphogypsum carbonation with ammonia under increased CO2 pressure.JOURNAL OF CO2 UTILIZATION,11(SEP),10-19. |
| MLA | Zhao, Hongtao,et al."Experimental study of enhanced phosphogypsum carbonation with ammonia under increased CO2 pressure".JOURNAL OF CO2 UTILIZATION 11.SEP(2015):10-19. |
入库方式： OAI收割
来源：过程工程研究所
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