Highly efficient and selective removal of trace lead from aqueous solutions by hollow mesoporous silica loaded with molecularly imprinted polymers
文献类型:期刊论文
作者 | Zhang, Zulei1,2; Zhang, Xingdi1; Niu, Dechao1; Li, Yongsheng1; Shi, Jianlin1,3 |
刊名 | JOURNAL OF HAZARDOUS MATERIALS
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出版日期 | 2017-04-15 |
卷号 | 328页码:160-169 |
关键词 | Hollow mesoporous silica Molecular imprinting Pb2+ Selectivity Real water sample |
英文摘要 | A novel type of adsorbent for the selective recognition and adsorption of trace Pb2+ from aqueous solutions has been successfully constructed simply by grafting molecularly imprinted polymers (MIPs) onto hollow mesoporous silica (HMS). Attractively, the HMS loaded with MIPs (H-MIPs) exhibits a fast adsorption kinetics, marked adsorption capacity of 40.52 mg/g and extremely high selectivity toward Pb2+ over Cu2+, Zn2+, Co2+, Mn2+ and Ni2+, and the selectivity coefficients have been determined to be as high as 50. Moreover, such high adsorptive capability and selectivity were retained for at least 6 runs, indicating the stability and reusability of H-MIPs. Lead ion contaminants in real water samples were successfully concentrated and approximately 100% recovered using H-MIPs. Theoretical analysis shows that the adsorption process of H-MIPs follows the pseudo-second-order kinetic and Langmuir isotherm models. These demonstrate that H-MIPs are greatly potential for the rapid and highly efficient removal of trace Pb2+ ions in complicated matrices. (C) 2017 Published by Elsevier B.V. |
WOS标题词 | Science & Technology ; Technology ; Life Sciences & Biomedicine |
类目[WOS] | Engineering, Environmental ; Engineering, Civil ; Environmental Sciences |
研究领域[WOS] | Engineering ; Environmental Sciences & Ecology |
关键词[WOS] | SOLID-PHASE EXTRACTION ; ADSORPTION PERFORMANCE ; FUNCTIONAL MONOMERS ; WATER SAMPLES ; PB(II) ; IONS ; CD(II) ; PRECONCENTRATION ; NANOPARTICLES ; CHEMISTRY |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000395228300018 |
源URL | [http://ir.sic.ac.cn/handle/331005/23716] ![]() |
专题 | 上海硅酸盐研究所_高性能陶瓷和超微结构国家重点实验室_期刊论文 |
作者单位 | 1.East China Univ Sci & Technol, Sch Mat Sci & Engn, Lab Low Dimens Mat Chem, Key Lab Ultrafine Mat Minist Educ, Shanghai 200237, Peoples R China 2.Jiaxing Univ, Sch Biol & Chem Engn, Jiaxing 314001, Peoples R China 3.Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Zulei,Zhang, Xingdi,Niu, Dechao,et al. Highly efficient and selective removal of trace lead from aqueous solutions by hollow mesoporous silica loaded with molecularly imprinted polymers[J]. JOURNAL OF HAZARDOUS MATERIALS,2017,328:160-169. |
APA | Zhang, Zulei,Zhang, Xingdi,Niu, Dechao,Li, Yongsheng,&Shi, Jianlin.(2017).Highly efficient and selective removal of trace lead from aqueous solutions by hollow mesoporous silica loaded with molecularly imprinted polymers.JOURNAL OF HAZARDOUS MATERIALS,328,160-169. |
MLA | Zhang, Zulei,et al."Highly efficient and selective removal of trace lead from aqueous solutions by hollow mesoporous silica loaded with molecularly imprinted polymers".JOURNAL OF HAZARDOUS MATERIALS 328(2017):160-169. |
入库方式: OAI收割
来源:上海硅酸盐研究所
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