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Atmospheric fossil fuel CO2 traced by (CO2)-C-14 and air quality index pollutant observations in Beijing and Xiamen, China

文献类型：期刊论文

作者Niu, Zhenchuan1,4,5; Zhou, Weijian1,3,4,5; Feng, Xue2; Feng, Tian1,5; Wu, Shugang1,5; Cheng, Peng1,5; Lu, Xuefeng1,5; Du, Hua1,5; Xiong, Xiaohu1,5; Fu, Yunchong1,5
刊名ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
出版日期2018-06-01
卷号25期号:17页码:17109-17117
关键词Delta C-14 Fossil Fuel Co2 Indirect Tracer Co Pm2.5
DOI10.1007/s11356-018-1616-z
文献子类Article
英文摘要Radiocarbon (C-14) is the most accurate tracer available for quantifying atmospheric CO2 derived from fossil fuel (CO2ff ), but it is expensive and time-consuming to measure. Here, we used common hourly Air Quality Index (AQI) pollutants (AQI, PM2.5, PM10, and CO) to indirectly trace diurnal CO2ff variations during certain days at the urban sites in Beijing and Xiamen, China, based on linear relationships between AQI pollutants and CO2ff traced by C-14 (CO2ff-C-14) for semimonthly samples obtained in 2014. We validated these indirectly traced CO2ff (CO2ff-in ) concentrations against CO2ff C-14 concentrations traced by simultaneous diurnal (CO2)-C-14 observations. Significant (p < 0.05) strong correlations were observed between each of the separate AQI pollutants and CO2ff-C-14 for the semimonthly samples. Diurnal variations in CO2ff traced by each of the AQI pollutants generally showed similar trends to those of CO2ff-C-14, with high agreement at the sampling site in Beijing and relatively poor agreement at the sampling site in Xiamen. AQI pollutant tracers showed high normalized root-mean-square (NRMS) errors for the summer diurnal samples due to low CO2ff-C-14 concentrations. After the removal of these summer samples, the NRMS errors for AQI pollutant tracers were in the range of 31.6-64.2%. CO generally showed a high agreement and low NRMS errors among these indirect tracers. Based on these linear relationships, monthly CO2ff averages at the sampling sites in Beijing and Xiamen were traced using CO concentration as a tracer. The monthly CO2ff averages at the Beijing site showed a shallow U-type variation. These results indicate that CO can be used to trace CO2ff variations in Chinese cities with CO2ff concentrations above 5 ppm.
WOS关键词LOS-ANGELES MEGACITY ; SOURCE APPORTIONMENT ; CARBON-DIOXIDE ; BACKGROUND SITES ; URBAN AREA ; EMISSIONS ; RADIOCARBON ; PM2.5 ; DELTA-C-14 ; EUROPE
WOS研究方向Environmental Sciences & Ecology
项目编号4177314、41573136、41730108 ; XAB2015A02 ; 2016360
WOS记录号WOS:000435961300079
资助机构the National Natural Science Foundation of China ; CAS“Light of West China” Program ; the Youth Innovation Promotion Association CAS
源URL[http://ir.ieecas.cn/handle/361006/5102]  
专题地球环境研究所_加速器质谱中心
作者单位1.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Shaanxi, Peoples R China
2.Northwest Univ, Coll Urban & Environm Sci, Xian, Shaanxi, Peoples R China
3.Beijing Normal Univ, Joint Ctr Global Change Studies, Beijing, Peoples R China
4.Qingdao Natl Lab Marine Sci & Technol, Open Studio Ocean Continental Climate & Environm, Qingdao, Peoples R China
5.Xian AMS Ctr, Shaanxi Key Lab Accelerator Mass Spectrometry Tec, Xian, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714		 Niu, Zhenchuan,Zhou, Weijian,Feng, Xue,et al. Atmospheric fossil fuel CO2 traced by (CO2)-C-14 and air quality index pollutant observations in Beijing and Xiamen, China[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2018,25(17):17109-17117.
APA Niu, Zhenchuan.,Zhou, Weijian.,Feng, Xue.,Feng, Tian.,Wu, Shugang.,...&Fu, Yunchong.(2018).Atmospheric fossil fuel CO2 traced by (CO2)-C-14 and air quality index pollutant observations in Beijing and Xiamen, China.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,25(17),17109-17117.
MLA Niu, Zhenchuan,et al."Atmospheric fossil fuel CO2 traced by (CO2)-C-14 and air quality index pollutant observations in Beijing and Xiamen, China".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 25.17(2018):17109-17117.

入库方式： OAI收割

来源：地球环境研究所

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