中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport

文献类型:期刊论文

作者Zhou, Jiamao; Zhao, ZZ(Zhao, Zhuzi)1; Cao, JJ(Cao, Junji)1; Ho, Steven Sai Hang1,2; Zhou, JM(Zhou, Jiamao)1,4; Tie, XX(Tie, Xuexi)1; Wang, P(Wang, Ping)3; Zhao, YZ(Zhao, Youzhi)3; Zhang, T(Zhang, Ting)1; Liu, SX(Liu, Suixin)1
刊名Environmental Science and Pollution Research
出版日期2018-07-01
卷号25期号:21页码:20591–20605
关键词Pm2.5 Chemical Composition Aerosol Acidity Regional Transport Sanya Organic Markers
DOI10.1007/s11356-018-2238-1
文献子类期刊论文
英文摘要An intensive sampling campaign of airborne fine particles (PM2.5) was conducted at Sanya, a coastal city in Southern China, from January to February 2012. Chemical analyses and mass reconstruction were used identify potential pollution sources and investigate atmospheric reaction mechanisms. A thermodynamic model indicated that low ammonia and high relative humidity caused the aerosols be acidic and that drove heterogeneous reactions which led to the formation of secondary inorganic aerosol. Relationships among neutralization ratios, free acidity, and air-mass trajectories suggest that the atmosphere at Sanya was impacted by both local and regional emissions. Three major transport pathways were identified, and flow from the northeast (from South China) typically brought the most polluted air to Sanya. A case study confirmed strong impact from South China (e.g., Pearl River Delta region) (contributed 76.8% to EC, and then this result can be extended to primary pollutants) when the northeast winds were dominant. The Weather Research Forecasting Black carbon model and trace organic markers were used to apportion local pollution versus regional contributions. Results of the study offer new insights into the atmospheric conditions and air pollution at this coastal city.
项目编号XDB05060500 ; 2013FY112700 ; 417151 ; RHDXB201613 ; RDJGb2016-18 ; Marine Geology-2017
语种英语
资助机构the project from theBStrategic Priority Research Program^ of the Chinese Academy of Science ; the project from theBStrategic Priority Research Program^ of the Chinese Academy of Science ; the project from Ministry of Science and Technology ; the project from Ministry of Science and Technology ; theNatural Science Foundation of Hainan Province, China ; theNatural Science Foundation of Hainan Province, China ; The Doctoral Scientific Research Foundation of Hainan Tropical Ocean University ; The Doctoral Scientific Research Foundation of Hainan Tropical Ocean University ; EducationalReform of Hainan Tropical Ocean University ; EducationalReform of Hainan Tropical Ocean University ; Key Discipline Construction Program of Hainan ProvincialDepartment of Education ; Key Discipline Construction Program of Hainan ProvincialDepartment of Education
源URL[http://ir.ieecas.cn/handle/361006/5259]  
专题地球环境研究所_粉尘与环境研究室
通讯作者Zhou, Jiamao
作者单位1.KLACP, SKLLQG, Institute of Earth Environment, ChineseAcademy of Sciences, Xi’an 710061, China
2.Division of Atmospheric Sciences, Desert Research Institute,Reno, NV 89512, USA
3.Hainan Tropical Ocean University, Sanya 572022, China
4.University of Chinese Academy of Sciences, Beijing 100049, China
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GB/T 7714
Zhou, Jiamao,Zhao, ZZ,Cao, JJ,et al. Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport[J]. Environmental Science and Pollution Research,2018,25(21):20591–20605.
APA Zhou, Jiamao.,Zhao, ZZ.,Cao, JJ.,Ho, Steven Sai Hang.,Zhou, JM.,...&Zhao, SY.(2018).Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport.Environmental Science and Pollution Research,25(21),20591–20605.
MLA Zhou, Jiamao,et al."Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport".Environmental Science and Pollution Research 25.21(2018):20591–20605.

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来源:地球环境研究所

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