Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport
文献类型:期刊论文
作者 | Zhou, Jiamao; Zhao, ZZ(Zhao, Zhuzi)1; Cao, JJ(Cao, Junji)1; Ho, Steven Sai Hang1,2; Zhou, JM(Zhou, Jiamao)1,4; Tie, XX(Tie, Xuexi)1; Wang, P(Wang, Ping)3; Zhao, YZ(Zhao, Youzhi)3; Zhang, T(Zhang, Ting)1; Liu, SX(Liu, Suixin)1 |
刊名 | Environmental Science and Pollution Research
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出版日期 | 2018-07-01 |
卷号 | 25期号:21页码:20591–20605 |
关键词 | Pm2.5 Chemical Composition Aerosol Acidity Regional Transport Sanya Organic Markers |
DOI | 10.1007/s11356-018-2238-1 |
文献子类 | 期刊论文 |
英文摘要 | An intensive sampling campaign of airborne fine particles (PM2.5) was conducted at Sanya, a coastal city in Southern China, from January to February 2012. Chemical analyses and mass reconstruction were used identify potential pollution sources and investigate atmospheric reaction mechanisms. A thermodynamic model indicated that low ammonia and high relative humidity caused the aerosols be acidic and that drove heterogeneous reactions which led to the formation of secondary inorganic aerosol. Relationships among neutralization ratios, free acidity, and air-mass trajectories suggest that the atmosphere at Sanya was impacted by both local and regional emissions. Three major transport pathways were identified, and flow from the northeast (from South China) typically brought the most polluted air to Sanya. A case study confirmed strong impact from South China (e.g., Pearl River Delta region) (contributed 76.8% to EC, and then this result can be extended to primary pollutants) when the northeast winds were dominant. The Weather Research Forecasting Black carbon model and trace organic markers were used to apportion local pollution versus regional contributions. Results of the study offer new insights into the atmospheric conditions and air pollution at this coastal city. |
项目编号 | XDB05060500 ; 2013FY112700 ; 417151 ; RHDXB201613 ; RDJGb2016-18 ; Marine Geology-2017 |
语种 | 英语 |
资助机构 | the project from theBStrategic Priority Research Program^ of the Chinese Academy of Science ; the project from theBStrategic Priority Research Program^ of the Chinese Academy of Science ; the project from Ministry of Science and Technology ; the project from Ministry of Science and Technology ; theNatural Science Foundation of Hainan Province, China ; theNatural Science Foundation of Hainan Province, China ; The Doctoral Scientific Research Foundation of Hainan Tropical Ocean University ; The Doctoral Scientific Research Foundation of Hainan Tropical Ocean University ; EducationalReform of Hainan Tropical Ocean University ; EducationalReform of Hainan Tropical Ocean University ; Key Discipline Construction Program of Hainan ProvincialDepartment of Education ; Key Discipline Construction Program of Hainan ProvincialDepartment of Education |
源URL | [http://ir.ieecas.cn/handle/361006/5259] ![]() |
专题 | 地球环境研究所_粉尘与环境研究室 |
通讯作者 | Zhou, Jiamao |
作者单位 | 1.KLACP, SKLLQG, Institute of Earth Environment, ChineseAcademy of Sciences, Xi’an 710061, China 2.Division of Atmospheric Sciences, Desert Research Institute,Reno, NV 89512, USA 3.Hainan Tropical Ocean University, Sanya 572022, China 4.University of Chinese Academy of Sciences, Beijing 100049, China |
推荐引用方式 GB/T 7714 | Zhou, Jiamao,Zhao, ZZ,Cao, JJ,et al. Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport[J]. Environmental Science and Pollution Research,2018,25(21):20591–20605. |
APA | Zhou, Jiamao.,Zhao, ZZ.,Cao, JJ.,Ho, Steven Sai Hang.,Zhou, JM.,...&Zhao, SY.(2018).Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport.Environmental Science and Pollution Research,25(21),20591–20605. |
MLA | Zhou, Jiamao,et al."Chemical characterization of PM2.5 from a southern coastal city of China:applications of modeling and chemical tracers in demonstrationof regional transport".Environmental Science and Pollution Research 25.21(2018):20591–20605. |
入库方式: OAI收割
来源:地球环境研究所
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