Simulations of organic aerosol concentrations during springtime in the Guanzhong Basin, China
文献类型：期刊论文
| 作者 | Feng, Tian4,5; Molina, Luisa T.1,2; Tie, Xuexi4; Huang, Ru-jin4; Wang, Yichen4; Zhang, Ting4; Liu, Suixin4; Zhou, Weijian4; Shen, Zhenxing3; Bei, Naifang4,5 |
| 刊名 | ATMOSPHERIC CHEMISTRY AND PHYSICS
 |
| 出版日期 | 2016-08-09 |
| 卷号 | 16期号:15页码:10045-10061 |
| DOI | 10.5194/acp-16-10045-2016 |
| 文献子类 | Article |
| 英文摘要 | The organic aerosol (OA) concentration is simulated in the Guanzhong Basin, China from 23 to 25 April 2013 utilizing the WRF-CHEM model. Two approaches are used to predict OA concentrations: (1) a traditional secondary organic aerosol (SOA) module; (2) a non-traditional SOA module including the volatility basis-set modeling method in which primary organic aerosol (POA) is assumed to be semivolatile and photochemically reactive. Generally, the spatial patterns and temporal variations of the calculated hourly near-surface ozone and fine particle matters agree well with the observations in Xi'an and surrounding areas. The model also yields reasonable distributions of daily PM2.5 and elemental carbon (EC) compared to the filter measurements at 29 sites in the basin. Filter-measured organic carbon (OC) and EC are used to evaluate OA, POA, and SOA using the OCaEuro-a center dot aEuro-EC ratio approach. Compared with the traditional SOA module, the non-traditional module significantly improves SOA simulations and explains about 88aEuro-% of the observed SOA concentration. Oxidation and partitioning of POA treated as semivolatile constitute the most important pathway for the SOA formation, contributing more than 75aEuro-% of the SOA concentrations in the basin. Residential emissions are the dominant anthropogenic OA source, constituting about 50aEuro-% of OA concentrations in urban and rural areas and 30aEuro-% in the background area. The OA contribution from transportation emissions decreases from 25aEuro-% in urban areas to 20aEuro-% in the background area, and the industry emission OA contribution is less than 6aEuro-%. |
| WOS关键词 | CHEMICAL-TRANSPORT MODEL ; RIVER DELTA REGION ; BASIS-SET APPROACH ; MEXICO-CITY BASIN ; METEOROLOGICAL UNCERTAINTIES ; MCMA-2006/MILAGRO CAMPAIGN ; SEMIVOLATILE ORGANICS ; SOURCE APPORTIONMENT ; SEASONAL-VARIATIONS ; INORGANIC AEROSOLS |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000383144600004 |
| 源URL | [http://ir.ieecas.cn/handle/361006/5692]  |
| 专题 | 地球环境研究所_粉尘与环境研究室 |
| 作者单位 | 1.MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA 02139 USA 2.Molina Ctr Energy & Environm, La Jolla, CA 92037 USA 3.Xi An Jiao Tong Univ, Sch Energy & Power Engn, Xian, Shaanxi, Peoples R China 4.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Key Lab Aerosol Chem & Phys, Xian, Peoples R China 5.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Shaanxi, Peoples R China |
| 推荐引用方式 GB/T 7714 | Feng, Tian,Molina, Luisa T.,Tie, Xuexi,et al. Simulations of organic aerosol concentrations during springtime in the Guanzhong Basin, China[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2016,16(15):10045-10061. |
| APA | Feng, Tian.,Molina, Luisa T..,Tie, Xuexi.,Huang, Ru-jin.,Wang, Yichen.,...&Li, Guohui.(2016).Simulations of organic aerosol concentrations during springtime in the Guanzhong Basin, China.ATMOSPHERIC CHEMISTRY AND PHYSICS,16(15),10045-10061. |
| MLA | Feng, Tian,et al."Simulations of organic aerosol concentrations during springtime in the Guanzhong Basin, China".ATMOSPHERIC CHEMISTRY AND PHYSICS 16.15(2016):10045-10061. |
入库方式： OAI收割
来源：地球环境研究所
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