中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Iodine isotopes in precipitation: Four-year time series variations before and after 2011 Fukushima nuclear accident

文献类型:期刊论文

作者Zhang, Luyuan2,4; Xu, Sheng1,3; Freeman, Stewart P. H. T.3; Hou, Xiaolin2; Watanabe, Akira1; Sanderson, David C. W.3; Cresswell, Alan1,3; Yamaguchi, Katsuhiko1
刊名JOURNAL OF ENVIRONMENTAL RADIOACTIVITY
出版日期2016-05-01
卷号155期号:2016页码:38-45
关键词Fukushima-derived I-129 I-129/i-127 Long-term Variation Rainwater Fukushima Nuclear Accident
DOI10.1016/j.jenvrad.2016.02.011
文献子类Article
英文摘要Rainwater samples were collected monthly from Fukushima, Japan, in 2012-2014 and analysed for I-127 and I-129. These are combined with previously reported data to investigate atmospheric levels and behaviour of Fukushima-derived I-129 before and after the 2011 nuclear accident. In the new datasets, I-127 and I-129 concentrations between October 2012 and October 2014 varied from 0.5 to 10 mu g/L and from 1.2 x 10(8) to 6.9 x 10(9) atoms/L respectively, resulting in I-129/I-127 atomic ratio ranges from 3 x 10(-8) to 2 x 10(-7). The I-129 concentrations were in good agreement with those in the previous period from March 2011 to September 2012, whereas the I-129 concentrations and I-129/I-127 ratios followed declining trends since the accident. Although I-129 concentrations in five samples during the period of 2013-2014 have approached the pre-accident levels, I-129 concentrations in most samples remained higher values in winter and spring-summer. The high I-129 levels in winter and spring-summer are most likely attributed to local resuspension of the Fukushima-derived radionuclide-bearing fine soil particles deposited on land surfaces, and re-emission through vegetation taking up I-129 from contaminated soil and water, respectively. Long-term declining rate suggests that contribution of the Fukushima-derived I-129 to the atmosphere would become less since 2014. (C) 2016 Elsevier Ltd. All rights reserved.
WOS关键词POWER-PLANT ACCIDENT ; REPROCESSING FACILITIES ; ENVIRONMENTAL-SAMPLES ; ATMOSPHERIC FALLOUT ; I-129 ; JAPAN ; SOIL ; RADIONUCLIDES ; CS-137 ; VOLATILIZATION
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000374358100006
源URL[http://ir.ieecas.cn/handle/361006/5761]  
专题地球环境研究所_加速器质谱中心
作者单位1.Fukushima Univ, Fukushima 9601296, Japan
2.Tech Univ Denmark, Ctr Nucl Technol, DK-4000 Roskilde, Denmark
3.Scottish Univ, Environm Res Ctr, E Kilbride G75 0QF, Lanark, Scotland
4.Chinese Acad Sci, Inst Earth Environm, Xian AMS Ctr, SKLLQG, Xian 710061, Peoples R China
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Zhang, Luyuan,Xu, Sheng,Freeman, Stewart P. H. T.,et al. Iodine isotopes in precipitation: Four-year time series variations before and after 2011 Fukushima nuclear accident[J]. JOURNAL OF ENVIRONMENTAL RADIOACTIVITY,2016,155(2016):38-45.
APA Zhang, Luyuan.,Xu, Sheng.,Freeman, Stewart P. H. T..,Hou, Xiaolin.,Watanabe, Akira.,...&Yamaguchi, Katsuhiko.(2016).Iodine isotopes in precipitation: Four-year time series variations before and after 2011 Fukushima nuclear accident.JOURNAL OF ENVIRONMENTAL RADIOACTIVITY,155(2016),38-45.
MLA Zhang, Luyuan,et al."Iodine isotopes in precipitation: Four-year time series variations before and after 2011 Fukushima nuclear accident".JOURNAL OF ENVIRONMENTAL RADIOACTIVITY 155.2016(2016):38-45.

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来源:地球环境研究所

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