Summertime ozone formation in Xi'an and surrounding areas, China
文献类型：期刊论文
| 作者 | Cao, Junji5,6; Zhou, Weijian5; Tie, Xuexi5,6; Liu, Suixin5,6; Zhang, Ting5,6; Su, Xiaoli5,6; Lei, Wenfang3; Molina, Luisa T.3; Li, Guohui5,6; Huang, Ru-Jin4,6 |
| 刊名 | ATMOSPHERIC CHEMISTRY AND PHYSICS
 |
| 出版日期 | 2016 |
| 卷号 | 16期号:7页码:4323-4342 |
| DOI | 10.5194/acp-16-4323-2016 |
| 文献子类 | Article |
| 英文摘要 | In this study, the ozone (O-3) formation in China's northwest city of Xi'an and surrounding areas is investigated using the Weather Research and Forecasting atmospheric chemistry (WRF-Chem) model during the period from 22 to 24 August 2013, corresponding to a heavy air pollution episode with high concentrations of O-3 and PM2.5. The model generally performs well compared to measurements in simulating the surface temperature, relative humidity, and wind speed and direction, near-surface O-3 and PM2.5 mass concentrations, and aerosol constituents. High aerosol concentrations in Xi'an and surrounding areas significantly decrease the photolysis frequencies and can reduce O-3 concentrations by more than 50 mu g m(-3) (around 25 ppb) on average. Sensitivity studies show that the O-3 production regime in Xi'an and surrounding areas is complicated, varying from NOx to VOC (volatile organic compound)-sensitive chemistry. The industrial emissions contribute the most to the O-3 concentrations compared to biogenic and other anthropogenic sources, but neither individual anthropogenic emission nor biogenic emission plays a dominant role in the O-3 formation. Under high O-3 and PM2.5 concentrations, a 50 % reduction in all the anthropogenic emissions only decreases near-surface O-3 concentrations by about 14 % during daytime. The complicated O-3 production regime and high aerosol levels pose a challenge for O-3 control strategies in Xi'an and surrounding areas. Further investigation regarding O-3 control strategies will need to be performed, taking into consideration the rapid changes in anthropogenic emissions that are not reflected in the current emission inventories and the uncertainties in the meteorological field simulations. |
| WOS关键词 | SECONDARY ORGANIC AEROSOL ; FINE PARTICULATE MATTER ; RIVER DELTA REGION ; MEXICO-CITY BASIN ; WRF-CHEM MODEL ; SURFACE OZONE ; FIELD CAMPAIGN ; AIR-QUALITY ; METEOROLOGICAL UNCERTAINTIES ; MCMA-2006/MILAGRO CAMPAIGN |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000374703000007 |
| 源URL | [http://ir.ieecas.cn/handle/361006/5772]  |
| 专题 | 地球环境研究所_粉尘与环境研究室 |
| 作者单位 | 1.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Peoples R China 2.Tsinghua Univ, Dept Environm Sci & Engn, Beijing 100084, Peoples R China 3.Molina Ctr Energy & Environm, La Jolla, CA USA 4.Paul Scherrer Inst, Lab Atmospher Chem, Villigen, Switzerland 5.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Peoples R China 6.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian, Peoples R China |
| 推荐引用方式 GB/T 7714 | Cao, Junji,Zhou, Weijian,Tie, Xuexi,et al. Summertime ozone formation in Xi'an and surrounding areas, China[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2016,16(7):4323-4342. |
| APA | Cao, Junji.,Zhou, Weijian.,Tie, Xuexi.,Liu, Suixin.,Zhang, Ting.,...&Zhang, Qiang.(2016).Summertime ozone formation in Xi'an and surrounding areas, China.ATMOSPHERIC CHEMISTRY AND PHYSICS,16(7),4323-4342. |
| MLA | Cao, Junji,et al."Summertime ozone formation in Xi'an and surrounding areas, China".ATMOSPHERIC CHEMISTRY AND PHYSICS 16.7(2016):4323-4342. |
入库方式： OAI收割
来源：地球环境研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。