Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow
文献类型：期刊论文
| 作者 | Lai, Senchao4,6; Zhao, Yan4; Zhang, Yingyi4; Fu, Pingqing3; Ho, Steven Sai Hang2,7; Wang, Shan4; Ho, Kin Fai1; Liu, Fobang6; Zou, Shichun5 |
| 刊名 | CHEMOSPHERE
 |
| 出版日期 | 2016-06-01 |
| 卷号 | 153期号:2016页码:332-339 |
| 关键词 | Northern South China Sea N-alkanes Pahs Hopanes Biomass Burning Long-range Transport |
| DOI | 10.1016/j.chemosphere.2016.03.069 |
| 文献子类 | Article |
| 英文摘要 | Filter samples of total suspended particle (TSP) collected during a cruise campaign over the northern South China Sea (SCS) from September to October 2013 were analyzed for non-polar organic compounds (NPOCs) as well as organic carbon (OC), elemental carbon (EC) and water-soluble ions. A total of 115 NPOCs species in groups of n-alkanes, polycyclic aromatic hydrocarbons (PAHs), iso-/antiso-alkanes, hopanes, steranes, methylalkanes, branched alkanes, cycloalkanes, alkenes and phthalates were detected. The characteristics of NPOCs in marine TSP samples were investigated to understand the sources from the Asian continent and other regions. The concentrations of total NPOCs ranged from 19.8 to 288.2 ng/m(3) with an average of 87.9 ng/m(3), which accounted for 0.8-1.7% (average 1.0%) of organic matter (OM). n-Alkanes was the predominant group, accounting for 43.1-79.5%, followed by PAHs (5.5-44.4%) and hopanes (1.6-11.4%). We found that primary combustion (biomass burning/fossil fuel combustion) was the dominant source for the majority of NPOCs (89.1%). Biomass burning in southern/southeastern China via long-range transport was proposed to be a major contributor of NPOCs in marine aerosols over the northern SCS, suggested by the significant correlations between nss-K+ and NPOCs groups as well as the analysis of air mass back-trajectory and fire spots. For the samples with strong continental influence, the strong enhancement in concentrations of n-alkanes, PAHs, hopanes and steranes were attributed to fossil fuel (coal/petroleum) combustion. In addition, terrestrial plants waxes were another contributor to NPOCs. (C) 2016 Elsevier Ltd. All rights reserved. |
| WOS关键词 | ATMOSPHERIC PARTICULATE MATTER ; MOLECULAR MARKER ; PACIFIC-OCEAN ; HONG-KONG ; TRACERS ; PAHS ; IDENTIFICATION ; TROPOSPHERE ; COMBUSTION ; DEPOSITION |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000375628800039 |
| 源URL | [http://ir.ieecas.cn/handle/361006/5786]  |
| 专题 | 地球环境研究所_黄土与第四纪地质国家重点实验室（2010~） |
| 作者单位 | 1.Chinese Univ Hong Kong, Jockey Club Sch Publ Hlth & Primary Care, Shatin, Hong Kong, Peoples R China 2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Peoples R China 3.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China 4.S China Univ Technol, Sch Environm & Energy, Guangdong Prov Key Lab Atmospher Environm & Pollu, Guangzhou 510641, Guangdong, Peoples R China 5.Sun Yat Sen Univ, Sch Marine Sci, Guangzhou 510275, Guangdong, Peoples R China 6.Max Planck Inst Chem, Multiphase Chem Dept, Mainz, Germany 7.Univ Nevada, Desert Res Inst, Div Atmospher Sci, 2215 Raggio Pathway, Reno, NV 89506 USA |
| 推荐引用方式 GB/T 7714 | Lai, Senchao,Zhao, Yan,Zhang, Yingyi,et al. Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow[J]. CHEMOSPHERE,2016,153(2016):332-339. |
| APA | Lai, Senchao.,Zhao, Yan.,Zhang, Yingyi.,Fu, Pingqing.,Ho, Steven Sai Hang.,...&Zou, Shichun.(2016).Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow.CHEMOSPHERE,153(2016),332-339. |
| MLA | Lai, Senchao,et al."Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow".CHEMOSPHERE 153.2016(2016):332-339. |
入库方式： OAI收割
来源：地球环境研究所
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