Resolving the impact of stratosphere-to-troposphere transport on the sulfur cycle and surface ozone over the Tibetan Plateau using a cosmogenic S-35 tracer
文献类型：期刊论文
| 作者 | Thiemens, Mark H.5; Chan, Chuen-Yu4; Kang, Shichang2,3,8; Zhang, Guoshuai1; Zhang, Qianggong1,8; Priyadarshi, Antra5; Hill-Falkenthal, Jason5; Su, Lin7; Zhang, Zhisheng6; Lin, Mang5 |
| 刊名 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
 |
| 出版日期 | 2016-01-16 |
| 卷号 | 121期号:1页码:439-456 |
| 关键词 | Radioactive Sulfur-35 Triple Oxygen Isotopes Stratosphere-troposphere Exchange Himalayas Nam Co Glacier Retreat |
| DOI | 10.1002/2015JD023801 |
| 文献子类 | Article |
| 英文摘要 | The Himalayas were recently identified as a global hot spot for deep stratosphere-to-troposphere transport (STT) in spring. Although the STT in this region may play a vital role in tropospheric chemistry, the hydrological cycle and aquatic ecosystems in Asia, there is no direct measurement of a chemical stratospheric tracer to verify and evaluate its possible impacts. Here we use cosmogenic S-35 as a tracer for air masses originating in the stratosphere and transported downward. We measure concentrations of S-35 in fresh surface snow and river runoff samples collected from Mount Everest in April 2013 to be more than 10 times higher than previously reported by any surface measurement, in support of the Himalayas as a gateway of springtime STT. In light of this result, measurements of (SO2)-S-35 and (SO42-)-S-35 at Nam Co in spring 2011 are reanalyzed to investigate the magnitudes of stratospheric air masses from the Himalayas to the tropospheric sulfur cycle and surface O-3 level over the Tibetan Plateau. A simple one-box model reveals that the oxidative lifetime of SO2 is reduced in aged STT plumes. Triple oxygen isotopic measurements of sulfate samples suggest that enhanced O-3 levels may shift the oxidation pathway of SO2 in the troposphere, which may be constrained by further intensive sampling and measurements. Comparison with surface O-3 measurements and traditional meteorological tracing methods shows that S-35 is a potentially unique and sensitive tracer to quantify the contribution of stratospheric air to surface O-3 levels in fresh or aged STT plumes. |
| WOS关键词 | DISPERSION MODEL FLEXPART ; SUMMER MONSOON SEASON ; ELEMENTAL COMPOSITION ; ATMOSPHERIC SULFATE ; DOWNWARD TRANSPORT ; MINERAL DUST ; BLACK-CARBON ; AIR-QUALITY ; SOUTH-ASIA ; NAM CO |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000369845300027 |
| 源URL | [http://ir.ieecas.cn/handle/361006/5821]  |
| 专题 | 地球环境研究所_黄土与第四纪地质国家重点实验室（2010~） |
| 作者单位 | 1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing, Peoples R China 2.Chinese Acad Sci, State Key Lab Cryospher Sci Cold & Arid Reg Envir, Lanzhou, Peoples R China 3.Chinese Acad Sci, Engn Res Inst, Lanzhou, Peoples R China 4.Chinese Acad Sci, Inst Earth Environm, Xian, Peoples R China 5.Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA 6.South China Inst Environm Sci, Minist Environm Protect, Guangzhou, Guangdong, Peoples R China 7.Hong Kong Univ Sci & Technol, Sch Sci, Environm Sci Programs, Hong Kong, Hong Kong, Peoples R China 8.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing, Peoples R China |
| 推荐引用方式 GB/T 7714 | Thiemens, Mark H.,Chan, Chuen-Yu,Kang, Shichang,et al. Resolving the impact of stratosphere-to-troposphere transport on the sulfur cycle and surface ozone over the Tibetan Plateau using a cosmogenic S-35 tracer[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2016,121(1):439-456. |
| APA | Thiemens, Mark H..,Chan, Chuen-Yu.,Kang, Shichang.,Zhang, Guoshuai.,Zhang, Qianggong.,...&Lin, Mang.(2016).Resolving the impact of stratosphere-to-troposphere transport on the sulfur cycle and surface ozone over the Tibetan Plateau using a cosmogenic S-35 tracer.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,121(1),439-456. |
| MLA | Thiemens, Mark H.,et al."Resolving the impact of stratosphere-to-troposphere transport on the sulfur cycle and surface ozone over the Tibetan Plateau using a cosmogenic S-35 tracer".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 121.1(2016):439-456. |
入库方式： OAI收割
来源：地球环境研究所
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