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Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste

文献类型：期刊论文

作者Lu, Xirui1,2; Shu, Xiaoyan1,2; Wang, Lan2; Shao, Dadong3; Zhang, Haibin4; Zhang, Kuibao1; Xie, Yi3
刊名JOURNAL OF ALLOYS AND COMPOUNDS
出版日期2019-01-15
卷号771页码:973-979
关键词Pyrochlore Gd2Zr2O7 TRPO waste Irradiation effects Phase transformation
ISSN号0925-8388
DOI10.1016/j.jallcom.2018.09.006
通讯作者Lu, Xirui(luxirui@swust.edu.cn) ; Zhang, Haibin(wsschbinzhang@163.com)
英文摘要The irradiation response of Gd2Zr2O7 ceramic bearing complex nuclear waste was explored by heavy ions to relatively high fluences. The Gd2Zr2O7 ceramic holding 25 wt.% and 40 wt.% of simulated TRPO waste (containing 11 kinds of oxides) were irradiated by 1.5 MeV Xe20+ to fluences ranging from 1.0 x 10(12) ions/cm(2) to 1.0 x 10(15) ions/cm(2) at room temperature. Irradiation induced structure disordering (i.e. phase transformation from pyrochlore to defect-fluorite and finally to amorphous structure) was disclosed by GIXRD, Raman and TEM. The results indicated the structure disordering was influenced by fluences, irradiation depth and waste loading content. This work identified the Gd2Zr2O7 ceramics as a potential candidate in immobilizing complex oxides from the aspect of irradiation tolerance. (c) 2018 Elsevier B.V. All rights reserved.
WOS关键词PYROCHLORE ; EXTRACTION ; AMORPHIZATION ; RADIONUCLIDES ; A(2)B(2)O(7) ; TRANSITION ; ACTINIDES ; PRESSURE ; DISORDER ; GD2TI2O7
资助项目National Natural Science Foundation of China, China[21507105] ; Key Project of Sichuan Education Department, China[15ZB0116] ; Longshan academic talent research supporting program of SWUST, China[18LZX312] ; Longshan academic talent research supporting program of SWUST, China[18LZX520]
WOS研究方向Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering
语种英语
WOS记录号WOS:000449621500120
出版者ELSEVIER SCIENCE SA
资助机构National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; 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Longshan academic talent research supporting program of SWUST, China
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/34307]  
专题合肥物质科学研究院_中科院等离子体物理研究所
通讯作者Lu, Xirui; Zhang, Haibin
作者单位1.Southwest Univ Sci & Technol, State Key Lab Environm Friendly Energy Mat, Mianyang 621010, Sichuan, Peoples R China
2.Southwest Univ Sci & Technol, Fundamental Sci Nucl Wastes & Environm Safety Lab, Mianyang 621010, Peoples R China
3.Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China
4.China Acad Engn Phys, Inst Nucl Phys & Chem, Mianyang 621900, Peoples R China
推荐引用方式
GB/T 7714		 Lu, Xirui,Shu, Xiaoyan,Wang, Lan,et al. Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2019,771:973-979.
APA Lu, Xirui.,Shu, Xiaoyan.,Wang, Lan.,Shao, Dadong.,Zhang, Haibin.,...&Xie, Yi.(2019).Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste.JOURNAL OF ALLOYS AND COMPOUNDS,771,973-979.
MLA Lu, Xirui,et al."Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste".JOURNAL OF ALLOYS AND COMPOUNDS 771(2019):973-979.

入库方式： OAI收割

来源：合肥物质科学研究院

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