中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Magnetic signatures of natural and anthropogenic sources of urban dust aerosol

文献类型:期刊论文

作者Liu, Haijiao2,3; Yan, Yan4; Chang, Hong2,7; Chen, Hongyun1; Liang, Lianji6; Liu, Xingxing2,7; Qiang, Xiaoke2,7; Sun, Youbin2,5,7
刊名ATMOSPHERIC CHEMISTRY AND PHYSICS
出版日期2019-01-21
卷号19期号:2页码:731-745
ISSN号1680-7316
DOI10.5194/acp-19-731-2019
通讯作者Sun, Youbin(sunyb@ieecas.cn)
英文摘要The characteristics of urban dust aerosols and the contributions of their natural and anthropogenic sources are of scientific interest as well as being of substantial sociopolitical and economic concern. Here we present a comprehensive study of dust flux, magnetic parameters, magnetic particulate morphology, and elemental compositions of atmospheric dustfall originating from natural dust sources in East Asia and local anthropogenic sources in Xi'an, China. The results reveal a significant inverse relationship between seasonal variations of dust flux and magnetic susceptibility (chi). By comparing dust flux and chi records, the relative contributions of dust from local anthropogenic sources are estimated. Analyses using scanning electron microscopy (SEM) combined with energy dispersive spectroscopy (EDS) indicate that magnetic particulate from different sources has distinct morphological and elemental characteristics. Detrital magnetic particles originating from natural sources are characterized by relatively smooth surfaces with Fe and O as the major elements and a minor contribution from Ti. The anthropogenic particles have angular, spherical, aggregate, and porous shapes with distinctive contributions from marker elements, including S, Cr, Cu, Zn, Ni, Mn, and Ca. Our results demonstrate that this multidisciplinary approach is effective in distinguishing dust particles derived from distant natural sources and local anthropogenic sources and for the quantitative assessment of contributions from the two end-members.
WOS关键词HEAVY-METAL POLLUTION ; PARTICULATE MATTER ; AIR-POLLUTION ; ASIAN DUST ; FLY-ASH ; SPATIAL VARIATION ; INDUSTRIAL SITES ; TRACE-ELEMENTS ; HAZE EVENTS ; STREET DUST
资助项目National Key Research and Development Program of China[2016YFA0601902] ; Open Foundation of State Key Laboratory of Loess and Quaternary Geology[SKLLQG1631]
WOS研究方向Meteorology & Atmospheric Sciences
语种英语
WOS记录号WOS:000456300700001
出版者COPERNICUS GESELLSCHAFT MBH
资助机构National Key Research and Development Program of China ; Open Foundation of State Key Laboratory of Loess and Quaternary Geology
源URL[http://ir.ieecas.cn/handle/361006/14404]  
专题地球环境研究所_古环境研究室
通讯作者Sun, Youbin
作者单位1.Chinese Acad Geol Sci, Res Ctr Loess & Global Changes, Inst Hydrogeol & Environm Geol, Shijiazhuang 050803, Hebei, Peoples R China
2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
3.Univ Chinese Acad Sci, Coll Earth Sci, Beijing 100049, Peoples R China
4.Chinese Acad Sci, Guangzhou Inst Geochem, Key Lab Ocean & Marginal Sea Geol, Guangzhou 510640, Guangdong, Peoples R China
5.Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710049, Shaanxi, Peoples R China
6.Beijing Univ Technol, Coll Architecture & Civil Engn, Beijing 100124, Peoples R China
7.Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714
Liu, Haijiao,Yan, Yan,Chang, Hong,et al. Magnetic signatures of natural and anthropogenic sources of urban dust aerosol[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(2):731-745.
APA Liu, Haijiao.,Yan, Yan.,Chang, Hong.,Chen, Hongyun.,Liang, Lianji.,...&Sun, Youbin.(2019).Magnetic signatures of natural and anthropogenic sources of urban dust aerosol.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(2),731-745.
MLA Liu, Haijiao,et al."Magnetic signatures of natural and anthropogenic sources of urban dust aerosol".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.2(2019):731-745.

入库方式: OAI收割

来源:地球环境研究所

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