中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Emission reduction effect on PM2.5, SO2 and NOx by using red mud as additive in clean coal briquetting

文献类型:期刊论文

作者Zhang, Yue2; Shen, Zhenxing2; Zhang, Bin2; Sun, Jian3; Zhang, Leiming1; Zhang, Tian2; Xu, Hongmei2; Bei, Naifang2; Tian, Jie4; Wang, Qiyuan4
刊名ATMOSPHERIC ENVIRONMENT
出版日期2020-02-15
卷号223页码:9
关键词Clean coal briquettes Red mud Emission reduction
ISSN号1352-2310
DOI10.1016/j.atmosenv.2019.117203
通讯作者Shen, Zhenxing(zxshen@mail.xjtu.edu.cn)
英文摘要Emissions of PM2.5 and trace gases from residential coal consumption for winter heating have caused severe air pollution in northern China. Clean coal briquettes can meet both demands of clean environment and residential heating. As a byproduct from the Bayer process, red mud has the potential to be used as briquettes additive, although its recycling procedure is challenging. In this study, red mud was used to replace the currently used calcium oxide as additive in coal briquetting. Twelve sets of combustion experiments were conducted for bituminous coal, anthracite coal and their briquettes, and each set of the experiment was repeated at least three times. Emission profiles of PM2.5, SO2 and NOx were recorded during experiments. The highest emission reduction rates for PM2.5, SO2 and NOx were achieved at red mud contents of 10%, 5% and 2.5%, respectively, for bituminous coal, and at 10%, 5% and 7.5%, respectively, for anthracite coal. The corresponding emission reduction rates were 37.5%, 25.8% and 61.9% for bituminous coal and 31.2%, 55.1% and 17.9% for anthracite coal. In addition, both SO2 and NOx emissions showed clear peaks during the initial-burning stage for the two kinds of coals, while SO2 emission for anthracite coal burning showed another peak during the char-burning stage. Benefit analysis was also conducted assuming all the currently used raw coals were replaced with clean coal briquettes in Shaanxi province. The overall reductions are 2270.46 (t) year(-1) for PM2.5, 1538.00 (t) year(-1) for SO2 and 2177.81 (t) year(-1) for NOx in the province. Results presented in this study highlight that development of clean energy policies, such as replacing bituminous coal and anthracite coal with clean coal briquettes, will be effective to improve the regional air quality.
WOS关键词TRACE GAS EMISSIONS ; FLUIDIZED-BED COMBUSTION ; PULVERIZED COAL ; HOUSEHOLD STOVES ; HYDROGEN-SULFIDE ; CALCIUM-OXIDE ; BAYER PROCESS ; FUEL USE ; BIOMASS ; NITROGEN
资助项目National Key R&D Program of China[2017YFCO212205] ; Natural Science Foundation of Shaanxi Province, China[2019JQ-386] ; China Postdoctoral Science Foundation[2019M653658]
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
语种英语
WOS记录号WOS:000517660200050
出版者PERGAMON-ELSEVIER SCIENCE LTD
资助机构National Key R&D Program of China ; Natural Science Foundation of Shaanxi Province, China ; China Postdoctoral Science Foundation
源URL[http://ir.ieecas.cn/handle/361006/12656]  
专题地球环境研究所_粉尘与环境研究室
通讯作者Shen, Zhenxing
作者单位1.Environm & Climate Change Canada, Sci & Technol Branch, Air Qual Res Div, Toronto, ON, Canada
2.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Peoples R China
3.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Peoples R China
4.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, SKLLQG, Xian 710061, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Yue,Shen, Zhenxing,Zhang, Bin,et al. Emission reduction effect on PM2.5, SO2 and NOx by using red mud as additive in clean coal briquetting[J]. ATMOSPHERIC ENVIRONMENT,2020,223:9.
APA Zhang, Yue.,Shen, Zhenxing.,Zhang, Bin.,Sun, Jian.,Zhang, Leiming.,...&Cao, Junji.(2020).Emission reduction effect on PM2.5, SO2 and NOx by using red mud as additive in clean coal briquetting.ATMOSPHERIC ENVIRONMENT,223,9.
MLA Zhang, Yue,et al."Emission reduction effect on PM2.5, SO2 and NOx by using red mud as additive in clean coal briquetting".ATMOSPHERIC ENVIRONMENT 223(2020):9.

入库方式: OAI收割

来源:地球环境研究所

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