Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts
文献类型：期刊论文
| 作者 | Chang, Tian1,2,3; Lu, Jiaqi2; Shen, Zhenxing1,2; Zhang, Bin2; Huang, Yu1; Cao, Junji1; Liu, Hongxia2; Veerapandian, Savita K. P.3; De Geyter, Nathalie3; Morent, Rino3 |
| 刊名 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
 |
| 出版日期 | 2019-08-14 |
| 卷号 | 58期号:32页码:14719-14728 |
| ISSN号 | 0888-5885 |
| DOI | 10.1021/acs.iecr.9b02668 |
| 通讯作者 | Shen, Zhenxing(zxshen@mail.xjtu.edu.cn) |
| 英文摘要 | A system combining nonthermal plasma (NTP) and catalysis using Mn-Co/HZSM-5 catalyst has been developed to promote the oxidation of acetaldehyde and reduce the production of ozone. The introduction of catalyst improved the oxidation of acetaldehyde and inhibited the generation of O-3 in comparison with the NTP alone system. The mixed MnCo/HZSM-5 catalyst demonstrated the highest catalytic activity among the various prepared catalysts, and this was ascribed to its crystalline structure, redox property, and adsorbed surface oxygen of the catalyst. The removal efficiency of acetaldehyde and COx yield were positively associated with the specific energy density (SED), and they were inversely related to the gas flow rate. Nevertheless, the energy yield was in negative correlation with the SED and in positive association with the gas flow rate. Moreover, the impact of different catalysts on the acceleration of acetaldehyde degradation in the hybrid system was discussed by developing a simple kinetic model. |
| WOS关键词 | MIXED OXIDES ; OXIDATION ; TOLUENE ; MN ; GAS ; DECOMPOSITION ; COMBUSTION ; PRODUCTS ; DEGRADATION ; SYSTEM |
| 资助项目 | project DepollutAir of Interreg V France-Wallonie-Vlaanderen ; National Science Foundation of China (NSFC)[41573138] ; State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, CAS[SKLLQG1616] ; China Scholarship Council (CSC)[201806280087] ; Hundred Talent Program of the Chinese Academy of Sciences |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| 出版者 | AMER CHEMICAL SOC |
| WOS记录号 | WOS:000481568600013 |
| 资助机构 | project DepollutAir of Interreg V France-Wallonie-Vlaanderen ; National Science Foundation of China (NSFC) ; State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, CAS ; China Scholarship Council (CSC) ; Hundred Talent Program of the Chinese Academy of Sciences |
| 源URL | [http://ir.ieecas.cn/handle/361006/13598]  |
| 专题 | 地球环境研究所_粉尘与环境研究室 |
| 通讯作者 | Shen, Zhenxing |
| 作者单位 | 1.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, SKLLQG, Xian 710049, Shaanxi, Peoples R China 2.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Shaanxi, Peoples R China 3.Univ Ghent, Res Unit Plasma Technol, Dept Appl Phys, Fac Engn & Architecture, Sint Pietersnieuwstr 41-B4, B-9000 Ghent, Belgium |
| 推荐引用方式 GB/T 7714 | Chang, Tian,Lu, Jiaqi,Shen, Zhenxing,et al. Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2019,58(32):14719-14728. |
| APA | Chang, Tian.,Lu, Jiaqi.,Shen, Zhenxing.,Zhang, Bin.,Huang, Yu.,...&Morent, Rino.(2019).Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,58(32),14719-14728. |
| MLA | Chang, Tian,et al."Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 58.32(2019):14719-14728. |
入库方式： OAI收割
来源：地球环境研究所
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