Characterization of PM2.5 source profiles from typical biomass burning of maize straw, wheat straw, wood branch, and their processed products (briquette and charcoal) in China
文献类型：期刊论文
| 作者 | Sun, Jian2,4; Shen, Zhenxing5; Zhang, Yue5; Zhang, Qian5; Lei, Yali5; Huang, Yu4; Niu, Xinyi1; Xu, Hongmei5; Cao, Junji4; Ho, Steven Sai Hang3 |
| 刊名 | ATMOSPHERIC ENVIRONMENT
 |
| 出版日期 | 2019-05-15 |
| 卷号 | 205页码:36-45 |
| 关键词 | Source profiles Biomass burning Briquette Charcoal Fuel processing |
| ISSN号 | 1352-2310 |
| DOI | 10.1016/j.atmosenv.2019.02.038 |
| 通讯作者 | Shen, Zhenxing(zxshen@mail.xjtu.edu.cn) |
| 英文摘要 | Chemical profiles from burning of raw biomass materials (i.e., maize straw, wheat straw and wood branch) and their processed products (i.e., briquette and charcoal) were determined with a customized cleaning stove in a combustion chamber. Inorganic species such as water-soluble ions and elements, and carbonaceous fractions including saccharide and polycyclic aromatic hydrocarbons (PAHs) in fine particulate matter (PM2.5) were quantified. Organic carbon (OC) was the highest fraction with a mass contribution to PM(2.5 )ranging from 17.65 +/- 0.15% to 40.17 +/- 3.83%. Potassium (K+) and chloride (Cl-) were the two most abundant water-soluble ions (4.31 +/- 1.57% and 3.05 +/- 1.29%, respectively). Most elements (e.g., heavy metals) had relatively low fractions ( < 0.01%) or below detection limit. For organics, levoglucosan averagely accounted for over 60% in total quantified saccharides, while 4-ring PAHs was the most dominant fraction. The proportions of OC, sum of quantified PAHs (EPAH5) and levoglucosan, as well as diagnostic ratios such as OC/element carbon (EC), K+/ EC, and sum of quantified saccharides (Sigma saccharides)/PM2.5 showed a characteristic descending order of raw fuels > briquette > charcoal. In comparison, charcoal burning had lower fractions of the organics since most volatile matters and moisture had been removed during carbonization. In addition, the similarities of chemical profiles from different bio-fuels burning were assessed by calculating the coefficient of divergence (CD) and their correlations. Relatively low CD (0.21-0.36) and high correlation (R > 0.97) suggest that the chemical profiles from straw and their briquettes were similar. However, the profiles from charcoal burning showed significant differences between their corresponding raw fuels (CDs = 0.26-0.47, R = 0.69-0.99) and also large variations from each other (CDs = 0.40-0.49, R < 0.90). The results of this study summarize that the processed fuels especially charcoals are unique in source apportionment and inventory studies. |
| WOS关键词 | POLYCYCLIC AROMATIC-HYDROCARBONS ; CHEMICAL SOURCE PROFILES ; FINE-PARTICLE EMISSIONS ; PARTICULATE MATTER ; GUANZHONG PLAIN ; AGRICULTURAL BIOMASS ; COMBUSTION ; WINTER ; PM10 ; XIAN |
| 资助项目 | National Key R&D Program of China[2017YFC0212205] ; Natural Science Foundation of Shaanxi Province, China[2016ZDJC-22] ; SKLLQG, Chinese Academy of Sciences[SKLLQG1616] ; SKLLQG, Chinese Academy of Sciences[SKLLQG1826] |
| WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000464478900005 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 资助机构 | National Key R&D Program of China ; Natural Science Foundation of Shaanxi Province, China ; SKLLQG, Chinese Academy of Sciences |
| 源URL | [http://ir.ieecas.cn/handle/361006/14129]  |
| 专题 | 地球环境研究所_粉尘与环境研究室 |
| 通讯作者 | Shen, Zhenxing |
| 作者单位 | 1.Chinese Univ Hong Kong, Jockey Club Sch Publ Hlth & Primary Care, Hong Kong, Peoples R China 2.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Shaanxi, Peoples R China 3.Desert Res Inst, Div Atmospher Sci, Reno, NV 89512 USA 4.Chinese Acad Sci, Inst Earth Environm, SKLLQG, Key Lab Aerosol Chem & Phys, Xian 710049, Shaanxi, Peoples R China 5.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Shaanxi, Peoples R China |
| 推荐引用方式 GB/T 7714 | Sun, Jian,Shen, Zhenxing,Zhang, Yue,et al. Characterization of PM2.5 source profiles from typical biomass burning of maize straw, wheat straw, wood branch, and their processed products (briquette and charcoal) in China[J]. ATMOSPHERIC ENVIRONMENT,2019,205:36-45. |
| APA | Sun, Jian.,Shen, Zhenxing.,Zhang, Yue.,Zhang, Qian.,Lei, Yali.,...&Li, Xuxiang.(2019).Characterization of PM2.5 source profiles from typical biomass burning of maize straw, wheat straw, wood branch, and their processed products (briquette and charcoal) in China.ATMOSPHERIC ENVIRONMENT,205,36-45. |
| MLA | Sun, Jian,et al."Characterization of PM2.5 source profiles from typical biomass burning of maize straw, wheat straw, wood branch, and their processed products (briquette and charcoal) in China".ATMOSPHERIC ENVIRONMENT 205(2019):36-45. |
入库方式： OAI收割
来源：地球环境研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。