Aerosol-photolysis interaction reduces particulate matter during wintertime haze events
文献类型:期刊论文
作者 | Wu, Jiarui2,4; Bei, Naifang3; Hu, Bo6; Liu, Suixin2,4; Wang, Yuan5; Shen, Zhenxing2; Li, Xia2,4; Liu, Lang2,4; Wang, Ruonan2,4; Liu, Zirui6 |
刊名 | PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA |
出版日期 | 2020-05-05 |
卷号 | 117期号:18页码:9755-9761 |
ISSN号 | 0027-8424 |
关键词 | particulate pollution aerosol-radiation interaction aerosol-photolysis interaction |
DOI | 10.1073/pnas.1916775117 |
通讯作者 | Li, Guohui(ligh@ieecas.cn) |
英文摘要 | Aerosol-radiation interaction (ARI) plays a significant role in the accumulation of fine particulate matter (PM2.5) by stabilizing the planetary boundary layer and thus deteriorating air quality during haze events. However, modification of photolysis by aerosol scattering or absorbing solar radiation (aerosol-photolysis interaction or API) alters the atmospheric oxidizing capacity, decreases the rate of secondary aerosol formation, and ultimately alleviates the ARI effect on PM2.5 pollution. Therefore, the synergetic effect of both ARI and API can either aggravate or even mitigate PM2.5 pollution. To test the effect, a fully coupled Weather Research and Forecasting (WRF)-Chem model has been used to simulate a heavy haze episode in North China Plain. Our results show that ARI contributes to a 7.8% increase in near-surface PM2.5. However, API suppresses secondary aerosol formation, and the combination of ARI and API results in only 4.8% net increase of PM2.5. Additionally, API increases the solar radiation reaching the surface and perturbs aerosol nucleation and activation to form cloud condensation nuclei, influencing aerosol-cloud interaction. The results suggest that API reduces PM2.5 pollution during haze events, but adds uncertainties in climate prediction. |
WOS关键词 | TIANJIN-HEBEI BTH ; MEXICO-CITY ; OPTICAL-PROPERTIES ; BLACK CARBON ; BROWN CARBON ; HONO SOURCES ; CHINA ; POLLUTION ; RADIATION ; EMISSIONS |
资助项目 | National Key RD Plan[2017YFC0210000] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB40030200] ; National Research Program for Key Issues in Air Pollution Control[DQGG0105] ; NSF[1560494] |
WOS研究方向 | Science & Technology - Other Topics |
语种 | 英语 |
出版者 | NATL ACAD SCIENCES |
WOS记录号 | WOS:000531067600023 |
资助机构 | National Key RD Plan ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Research Program for Key Issues in Air Pollution Control ; NSF |
源URL | [http://ir.ieecas.cn/handle/361006/14748] |
专题 | 地球环境研究所_粉尘与环境研究室 第四纪科学与全球变化卓越创新中心 |
通讯作者 | Li, Guohui |
作者单位 | 1.Molina Ctr Energy & Environm, La Jolla, CA 92037 USA 2.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China 3.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Shaanxi, Peoples R China 4.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China 5.CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA 6.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China |
推荐引用方式 GB/T 7714 | Wu, Jiarui,Bei, Naifang,Hu, Bo,et al. Aerosol-photolysis interaction reduces particulate matter during wintertime haze events[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2020,117(18):9755-9761. |
APA | Wu, Jiarui.,Bei, Naifang.,Hu, Bo.,Liu, Suixin.,Wang, Yuan.,...&Li, Guohui.(2020).Aerosol-photolysis interaction reduces particulate matter during wintertime haze events.PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,117(18),9755-9761. |
MLA | Wu, Jiarui,et al."Aerosol-photolysis interaction reduces particulate matter during wintertime haze events".PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 117.18(2020):9755-9761. |
入库方式: OAI收割
来源:地球环境研究所
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