Characteristics of indoor and personal exposure to particulate organic compounds emitted from domestic solid fuel combustion in rural areas of northwest China
文献类型：期刊论文
| 作者 | He, Kailai2; Xu, Hongmei2,3; Feng, Rong2; Shen, Zhenxing2; Li, Yaqi2; Zhang, Yue2; Sun, Jian2; Zhang, Qian4; Zhang, Tian2; Yang, Liu2 |
| 刊名 | ATMOSPHERIC RESEARCH
 |
| 出版日期 | 2021-01-15 |
| 卷号 | 248页码:10 |
| ISSN号 | 0169-8095 |
| 关键词 | Personal exposure Indoor air pollution Domestic solid fuel Organic compounds Size distribution Health risk |
| DOI | 10.1016/j.atmosres.2020.105181 |
| 通讯作者 | Xu, Hongmei(xuhongmei@xjtu.edu.cn) |
| 英文摘要 | Household solid fuel combustion for heating in winter is a substantial source of air pollution in rural areas of northwest China. The present study investigated the concentration characteristics and health risks of particulate matter (PM) and its organic compounds, including polycyclic aromatic hydrocarbons (PAHs), oxygenated PAHs (OPAHs), and phthalate esters (PAEs). Indoor air and housewives' personal exposure (PE) samples were collected in Guanzhong Basin, among rural households relying on various solid fuels for heating in winter. Indoor PM primarily comprised fine PM (PM2.5, 76%), and its organic compounds were identified in particular abundance in households that used coal as the only domestic fuel (Group C, 96% in PM2.5). The mean concentration of PE to PM2.5 was 307 +/- 120 mu g center dot m(-3), which was 2.4-times higher than the indoor concentration (130 +/- 103 mu g center dot m(-3)) because of the housewives' short-term exposure to high-concentration pollution emitted by solid fuel combustion. Organic compounds exhibited the same pattern, with PE samples having a 44% higher concentration than indoor samples. The correlation of PM2.5-bound organics between indoor and PE samples in Group C (R-2 = 0.9) was higher than that in the group using coal and biomass (Group M, R-2 = 0.6), indicating the stronger correlation of single-fuel heating method. The PE/indoor ratio of high molecular weight (HMW) PAHs in Group C (2.5) was higher than that of the other organic compounds (1.3) because HMW PAHs emitted through coal combustion had a larger effect on PE. This further led to higher incremental lifetime cancer risks (ICLRs) via inhalation pathway among housewives in Group C (2.4 and 1.2-times higher risk for PAHs and PAEs, respectively) than among those in Group M. However, inhalational ILCR values of Group M were still 2.1-340-times higher than the international safety standard (10(-6)). Therefore, the upgradation of domestic fuels and heating ways is urgently needed in rural area of northwest China to reduce indoor air pollution and health risks. |
| WOS关键词 | POLYCYCLIC AROMATIC-HYDROCARBONS ; LUNG-CANCER RISK ; PORT THERMAL-DESORPTION ; HOUSEHOLD AIR-POLLUTION ; GUANZHONG PLAIN ; SIZE DISTRIBUTIONS ; EMISSION FACTORS ; HEALTH-RISK ; SPATIAL-DISTRIBUTION ; PM EXPOSURE |
| 资助项目 | National Natural Science Foundation of China[41877376] ; Key Project of Natural Science Basic Research Program of Shaanxi Province[2019JZ-36] ; Key Research and Development Program of Shaanxi Province[2018-ZDXM3-01] |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| 出版者 | ELSEVIER SCIENCE INC |
| WOS记录号 | WOS:000594097000006 |
| 资助机构 | National Natural Science Foundation of China ; Key Project of Natural Science Basic Research Program of Shaanxi Province ; Key Research and Development Program of Shaanxi Province |
| 源URL | [http://ir.ieecas.cn/handle/361006/15605]  |
| 专题 | 地球环境研究所_粉尘与环境研究室 |
| 通讯作者 | Xu, Hongmei |
| 作者单位 | 1.Chinese Univ Hong Kong, JC Sch Publ Hlth & Primary Care, Hong Kong, Peoples R China 2.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian, Peoples R China 3.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, SKLLQG, Xian, Peoples R China 4.Xian Univ Architecture & Technol, Sch Environm & Municipal Engn, Xian, Peoples R China |
| 推荐引用方式 GB/T 7714 | He, Kailai,Xu, Hongmei,Feng, Rong,et al. Characteristics of indoor and personal exposure to particulate organic compounds emitted from domestic solid fuel combustion in rural areas of northwest China[J]. ATMOSPHERIC RESEARCH,2021,248:10. |
| APA | He, Kailai.,Xu, Hongmei.,Feng, Rong.,Shen, Zhenxing.,Li, Yaqi.,...&Cao, Junji.(2021).Characteristics of indoor and personal exposure to particulate organic compounds emitted from domestic solid fuel combustion in rural areas of northwest China.ATMOSPHERIC RESEARCH,248,10. |
| MLA | He, Kailai,et al."Characteristics of indoor and personal exposure to particulate organic compounds emitted from domestic solid fuel combustion in rural areas of northwest China".ATMOSPHERIC RESEARCH 248(2021):10. |
入库方式： OAI收割
来源：地球环境研究所
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