Rapid solidification of Sr-contaminated soil by consecutive microwave sintering: mechanism and stability evaluation
文献类型:期刊论文
作者 | Tang, Hexi1,2; Shu, Xiaoyan3,4; Huang, Wenxiao5; Miao, Yulong4; Shi, Minghe4; Chen, Shunzhang6; Li, Bingsheng1,3; Luo, Fen3,4; Xie, Yi7,8; Shao, Dadong9 |
刊名 | JOURNAL OF HAZARDOUS MATERIALS |
出版日期 | 2021-04-05 |
卷号 | 407 |
ISSN号 | 0304-3894 |
关键词 | Sr-contaminated soil Consecutive microwave sintering Glass-ceramic Slawsonite Chemical durability |
DOI | 10.1016/j.jhazmat.2020.124761 |
通讯作者 | Lu, Xirui(luxiruimvp116@163.com) |
英文摘要 | Consecutive microwave sintering is a method proposed in this study to dispose soil contaminated by Sr during a nuclear accident by rapidly solidifying the contaminated soil. The results show that soil contaminated with 20 wt % SrSO4 and 30 wt% SrSO4 can be completely solidified by microwave sintering at 1100-1200 and 1300 degrees C, respectively, for 30 min. Sr was found to be cured into slawsonite (SrAl2Si2O8) and glass structures. Moreover, soil sintered at 1300 degrees C has large cured solubility (30 wt.%), good uniformity, and excellent hardness (6.9-7.2 GPa) and chemical durability (below 1.46 x 10(-5) g m(2) d(-1) at 28 d). Thus, consecutive microwave sintering technology may provide a new method for treating Sr-contaminated soil in case of a nuclear accident emergency. |
WOS关键词 | IMMOBILIZATION ; WASTE |
资助项目 | National Natural Science Foundation of China[21677118] ; Project of State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology[18fksy0213] ; Research Fund Program of Guangdong Key Laboratory of Radioactive and Rare Resource Utilization[2019-LRRRU02] |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | ELSEVIER |
WOS记录号 | WOS:000613429600006 |
资助机构 | National Natural Science Foundation of China ; Project of State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology ; Research Fund Program of Guangdong Key Laboratory of Radioactive and Rare Resource Utilization |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/120460] |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Lu, Xirui |
作者单位 | 1.Southwest Univ Sci & Technol, State Key Lab Environm Friendly Energy Mat, Mianyang 621010, Sichuan, Peoples R China 2.Sichuan Radiat Detect & Protect Inst Nucl Ind, Chengdu 610052, Peoples R China 3.Southwest Univ Sci & Technol, Natl Coinnovat Ctr Nucl Waste Disposal & Environm, Mianyang 621010, Sichuan, Peoples R China 4.Southwest Univ Sci & Technol, Fundamental Sci Nucl Wastes & Environm Safety Lab, Mianyang 621010, Sichuan, Peoples R China 5.Guangdong Prov Key Lab Radioact & Rare Resource U, Shaoguan 512026, Peoples R China 6.Sichuan Univ, Inst Nucl Sci & Technol, Chengdu 610064, Peoples R China 7.Univ Sci & Technol China, Hefei 230026, Peoples R China 8.Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China 9.Nanjing Univ Sci & Technol, Nanjing 210094, Peoples R China |
推荐引用方式 GB/T 7714 | Tang, Hexi,Shu, Xiaoyan,Huang, Wenxiao,et al. Rapid solidification of Sr-contaminated soil by consecutive microwave sintering: mechanism and stability evaluation[J]. JOURNAL OF HAZARDOUS MATERIALS,2021,407. |
APA | Tang, Hexi.,Shu, Xiaoyan.,Huang, Wenxiao.,Miao, Yulong.,Shi, Minghe.,...&Lu, Xirui.(2021).Rapid solidification of Sr-contaminated soil by consecutive microwave sintering: mechanism and stability evaluation.JOURNAL OF HAZARDOUS MATERIALS,407. |
MLA | Tang, Hexi,et al."Rapid solidification of Sr-contaminated soil by consecutive microwave sintering: mechanism and stability evaluation".JOURNAL OF HAZARDOUS MATERIALS 407(2021). |
入库方式: OAI收割
来源:合肥物质科学研究院
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