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Vapor isotopic evidence for the worsening of winter air quality by anthropogenic combustion-derived water

文献类型：期刊论文

作者Xing, Meng1,2; Liu, Weiguo1,2; Li, Xia1,3; Zhou, Weijian1,2,4; Wang, Qiyuan1,2,3; Tian, Jie1,2,3; Li, Xiaofei1,2,3; Tie, Xuexi1,2,3; Li, Guohui1,2,3; Cao, Junji1,2,3,5,6
刊名PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
出版日期2020-12-29
卷号117期号:52页码:33005-33010
关键词water vapor isotopes WRF-Chem simulation air quality winter haze
ISSN号0027-8424
DOI10.1073/pnas.1922840117
通讯作者Cao, Junji(jjcao@ieecas.cn) ; Bao, Huiming(bao@lsu.edu) ; An, Zhisheng(anzs@loess.llqg.ac.cn)
英文摘要Anthropogenic combustion-derived water (CDW) may accumulate in an airshed due to stagnant air, which may further enhance the formation of secondary aerosols and worsen air quality. Here we collected three-winter-season, hourly resolution, water-vapor stable H and O isotope compositions together with atmospheric physical and chemical data from the city of Xi'an, located in the Guanzhong Basin (GZB) in northwestern China, to elucidate the role of CDW in particulate pollution. Based on our experimentally determined water vapor isotope composition of the CDW for individual and weighted fuels in the basin, we found that CDW constitutes 6.2% of the atmospheric moisture on average and its fraction is positively correlated with [PM2.5] (concentration of particulate matter with an aerodynamic diameter less than 2.5 mu m) as well as relative humidity during the periods of rising [PM2.5]. Our modeling results showed that CDW added additional average 4.6 mu g m(-3) PM2.5 during severely polluted conditions in the GZB, which corresponded to an average 5.1% of local anthropogenic [PM2.5] (average at similar to 91.0 mu g m(-3)). Our result is consistent with the proposed positive feedback between the relative humidity and a moisture sensitive air-pollution condition, alerting to the nontrivial role of CDW when considering change of energy structure such as a massive coal-to-gas switch in household heating in winter.
WOS关键词MEXICO-CITY ; PARTICULATE MATTER ; DEUTERIUM EXCESS ; GUANZHONG BASIN ; HAZE ; POLLUTION ; EMISSIONS ; CHINA ; PM2.5 ; PHOTOCHEMISTRY
资助项目Strategic Priority Research Program of Chinese Academy of Sciences[XDB40000000] ; National Research Program for Key Issues in Air Pollution Control (China) Grant[DQGG0105] ; National Atmospheric Research Program (China) Grant[2017YFC0212200] ; Key Projects of Chinese Academy of Sciences Grant[ZDRW-ZS-2017-6] ; State Key Laboratory of Loess and Quaternary Geology Grant[SKLLQGZD1701] ; China scholarship council ; Charles Jones Professorship fund
WOS研究方向Science & Technology - Other Topics
语种英语
WOS记录号WOS:000604551600030
出版者NATL ACAD SCIENCES
资助机构Strategic Priority Research Program of Chinese Academy of Sciences ; National Research Program for Key Issues in Air Pollution Control (China) Grant ; National Atmospheric Research Program (China) Grant ; Key Projects of Chinese Academy of Sciences Grant ; State Key Laboratory of Loess and Quaternary Geology Grant ; China scholarship council ; Charles Jones Professorship fund
源URL[http://ir.ieecas.cn/handle/361006/15762]  
专题地球环境研究所_加速器质谱中心
第四纪科学与全球变化卓越创新中心
通讯作者Cao, Junji; Bao, Huiming; An, Zhisheng
作者单位1.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Peoples R China
2.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Peoples R China
3.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Peoples R China
4.Beijing Normal Univ, Interdisciplinary Res Ctr Earth Sci Frontier, Beijing 100875, Peoples R China
5.Qingdao Natl Lab Marine Sci & Technol, Open Studio Ocean Continental Climate & Environm, Qingdao, Peoples R China
6.Xi An Jiao Tong Univ, Dept Earth & Environm Sci, Xian 710049, Peoples R China
7.Nanjing Univ, Int Ctr Isotope Effects Res, Sch Earth Sci & Engn, Nanjing 210023, Peoples R China
8.Louisiana State Univ, Dept Geol & Geophys, Baton Rouge, LA 70803 USA
推荐引用方式
GB/T 7714		 Xing, Meng,Liu, Weiguo,Li, Xia,et al. Vapor isotopic evidence for the worsening of winter air quality by anthropogenic combustion-derived water[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2020,117(52):33005-33010.
APA Xing, Meng.,Liu, Weiguo.,Li, Xia.,Zhou, Weijian.,Wang, Qiyuan.,...&An, Zhisheng.(2020).Vapor isotopic evidence for the worsening of winter air quality by anthropogenic combustion-derived water.PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,117(52),33005-33010.
MLA Xing, Meng,et al."Vapor isotopic evidence for the worsening of winter air quality by anthropogenic combustion-derived water".PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 117.52(2020):33005-33010.

入库方式： OAI收割

来源：地球环境研究所

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