Characteristics and sources of amine-containing particles in the urban atmosphere of Liaocheng, a seriously polluted city in North China during the COVID-19 outbreak
文献类型：期刊论文
| 作者 | Li, Zheng1; Zhou, Ruiwen1; Wang, Yiqiu2; Wang, Gehui3; Chen, Min1; Li, Yuanyuan1; Wang, Yachen1; Yi, Yanan1; Hou, Zhanfang1; Guo, Qingchun1 |
| 刊名 | ENVIRONMENTAL POLLUTION
 |
| 出版日期 | 2021-11-15 |
| 卷号 | 289页码:10 |
| ISSN号 | 0269-7491 |
| 关键词 | Amine-containing particles Diethylamine (DEA) Gas-to-particle partitioning Air quality COVID-19 lockdown |
| DOI | 10.1016/j.envpol.2021.117887 |
| 通讯作者 | Meng, Jingjing(mengjingjing@lcu.edu.cn) |
| 英文摘要 | The Chinese government issued an unprecedentedly strict lockdown policy to control the spread of the novel coronavirus disease 2019 (COVID-19), significantly mitigating air pollution because of the dramatic reduction of industrial and traffic emissions. To explore the impact of COVID-19 lockdown (LCD) on organic aerosols, the mixing states and evolution processes of amine-containing particles were studied using a single particle aerosol mass spectrometer from January to March 2020 in Liaocheng, which is a seriously polluted city in North China. The counts and percentages of amine-containing particles in total obtained particles during the pre-LCD (547832, 29.8 %) were higher than those during the LCD (283983, 20.7 %) and post-LCD (102026, 18.4 %), mainly due to the reduced emission strength of amines and suppressed gas-to-particle partitioning of amines during the LCD and post-LCD. (74)(C2H5)(2)NH2+ was the most abundant amine marker, which accounted for 98.2 %, 98.4 %, and 96.7 % of all amine-containing particles during the pre-LCD, LCD, and post-LCD, respectively. Correlation analysis and temporal variations indicated that the gas-to-particle partitioning of amines was facilitated by the stronger acidic environment and lower temperature, while the effect of RH and aerosol liquid water content was minor. The A-OC particles were the most abundant type (accounting for similar to 40 %) throughout the observation period. The temporal profiles and correlation analysis suggested that the impact of the increased O-3 on the amines and their oxidation products (e.g., trimethylamine oxide) was minor. The identified particle types, correlation analysis, and the potential source contribution function results implied that the amine-containing particles were mainly derived from local and surrounding sources during the LCD, while those were mainly affected by long-range transport during the pre-LCD and post-LCD. Our results could deepen the comprehension of the sources and atmospheric processing of amines in the urban area of North China during the COVID-19 outbreak. |
| WOS关键词 | SECONDARY AEROSOL FORMATION ; WATER-SOLUBLE IONS ; PEARL RIVER-DELTA ; SINGLE-PARTICLE ; SULFURIC-ACID ; AMBIENT AEROSOL ; MIXING STATE ; AIR-QUALITY ; RURAL SITE ; PM2.5 |
| 资助项目 | National Science Foundation of China[41505112] ; National Science Foundation of China[41702373] ; Natural Science Foundation of Shandong Province[ZR2020MD113] ; Open Funds of State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences[SKLLQG2020] |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| 出版者 | ELSEVIER SCI LTD |
| WOS记录号 | WOS:000697053600008 |
| 资助机构 | National Science Foundation of China ; Natural Science Foundation of Shandong Province ; Open Funds of State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences |
| 源URL | [http://ir.ieecas.cn/handle/361006/17025]  |
| 专题 | 地球环境研究所_黄土与第四纪地质国家重点实验室（2010~） |
| 通讯作者 | Meng, Jingjing |
| 作者单位 | 1.Liaocheng Univ, Sch Geog & Environm, Liaocheng 252000, Shandong, Peoples R China 2.Liaocheng Environm Informat & Monitoring Ctr, Liaocheng 252000, Shandong, Peoples R China 3.East China Normal Univ, Sch Geog Sci, Key Lab Geog Informat Sci, Minist Educ, Shanghai 200062, Peoples R China 4.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, State Key Lab Loess & Quaternary Geol, Xian 710075, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Zheng,Zhou, Ruiwen,Wang, Yiqiu,et al. Characteristics and sources of amine-containing particles in the urban atmosphere of Liaocheng, a seriously polluted city in North China during the COVID-19 outbreak[J]. ENVIRONMENTAL POLLUTION,2021,289:10. |
| APA | Li, Zheng.,Zhou, Ruiwen.,Wang, Yiqiu.,Wang, Gehui.,Chen, Min.,...&Meng, Jingjing.(2021).Characteristics and sources of amine-containing particles in the urban atmosphere of Liaocheng, a seriously polluted city in North China during the COVID-19 outbreak.ENVIRONMENTAL POLLUTION,289,10. |
| MLA | Li, Zheng,et al."Characteristics and sources of amine-containing particles in the urban atmosphere of Liaocheng, a seriously polluted city in North China during the COVID-19 outbreak".ENVIRONMENTAL POLLUTION 289(2021):10. |
入库方式： OAI收割
来源：地球环境研究所
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