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Sediment Soot Radiocarbon Indicates that Recent Pollution Controls Slowed Fossil Fuel Emissions in Southeastern China

文献类型：期刊论文

作者Han, Yongming1,2,7; An, Zhisheng7; Arimoto, Richard7; Waters, Colin N.6; Schneider, Tobias4,5; Yao, Peng3; Sarli, Eirini3; Zhou, Weijian7; Li, Li7; Dusek, Ulrike3
刊名ENVIRONMENTAL SCIENCE & TECHNOLOGY
出版日期2022-01-10
页码10
ISSN号0013-936X
关键词fossil fuel usage black carbon human emissions pollution history lake sediments
DOI10.1021/acs.est.1c05424
通讯作者Han, Yongming(yongming@ieecas.cn) ; Dusek, Ulrike(u.dusek@rug.nl)
英文摘要Fossil fuel (FF) combustion emissions account for a large, but uncertain, amount of the soot in the atmosphere, play an important role in climate change, and adversely affect human health. However, historical estimates of FF contributions to air pollution are limited by uncertainties in fuel usage and emission factors. Here, we constrained FF soot emissions from southeastern China over the past 110 years, based on a novel radiocarbon method applied to sedimentary soot. The reconstructed soot accumulations reflect the integrated effects of increased FF use caused by economic development and reductions in emissions due to pollution controls. A sharp increase in FF soot started in 1950 as southeastern China industrialized and developed economically, but decreased FF soot fluxes in recent years suggest that pollution controls reduced soot emissions. We compare FF soot history to changes in CO2 emissions, industrial and economic activities, and pollution controls and show that FF soot fluxes are more readily controlled than atmospheric CO2. Our independent FF soot record provides insights into the effects of economic development and controls on air pollution and the environmental impacts from the changes in soot emissions.
WOS关键词REGIONAL BACKGROUND SITE ; BLACK CARBON EMISSIONS ; SOURCE APPORTIONMENT ; AEROSOLS ; INVENTORY ; BIOMASS ; MICADAS ; HAZE ; CHAR ; XIAN
资助项目NSFC[41625015] ; NSFC[41991250] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB40000000] ; Chinese Academy of Sciences[132B61KYSB20170005] ; SNSF[184428] ; China Scholarships Council[201806320346] ; HGY Scenic Spot Management Bureau
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000743227700001
资助机构NSFC ; Strategic Priority Research Program of Chinese Academy of Sciences ; Chinese Academy of Sciences ; SNSF ; China Scholarships Council ; HGY Scenic Spot Management Bureau
源URL[http://ir.ieecas.cn/handle/361006/17387]  
专题地球环境研究所_粉尘与环境研究室
第四纪科学与全球变化卓越创新中心
通讯作者Han, Yongming; Dusek, Ulrike
作者单位1.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Peoples R China
2.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Peoples R China
3.Energy & Sustainabil Res Inst Groningen ESRIG, Ctr Isotope Res CIO, NL-9747 AG Groningen, Netherlands
4.Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY 10964 USA
5.Univ Massachusetts, Dept Geosci, Morrill Sci Ctr, Amherst, MA 01003 USA
6.Univ Leicester, Sch Geog Geol & Environm, Leicester LE1 7RH, Leics, England
7.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Inst Earth Environm, SKLLQG, Xian 710061, Peoples R China
推荐引用方式
GB/T 7714		 Han, Yongming,An, Zhisheng,Arimoto, Richard,et al. Sediment Soot Radiocarbon Indicates that Recent Pollution Controls Slowed Fossil Fuel Emissions in Southeastern China[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2022:10.
APA Han, Yongming.,An, Zhisheng.,Arimoto, Richard.,Waters, Colin N..,Schneider, Tobias.,...&Dusek, Ulrike.(2022).Sediment Soot Radiocarbon Indicates that Recent Pollution Controls Slowed Fossil Fuel Emissions in Southeastern China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,10.
MLA Han, Yongming,et al."Sediment Soot Radiocarbon Indicates that Recent Pollution Controls Slowed Fossil Fuel Emissions in Southeastern China".ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022):10.

入库方式： OAI收割

来源：地球环境研究所

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