Radiocarbon in the Atmosphere and Seawater in the South China Sea: Flux, Inventory and Air-Sea CO2 Exchange Rate Tracing
文献类型:期刊论文
作者 | Niu, Zhenchuan2,3,4,5; Zhou, Weijian3,4,5; Zhao, Huiyizhe3,5; Feng, Xue1,5; Lyu, Mengni1,5 |
刊名 | JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES |
出版日期 | 2022-03-01 |
卷号 | 127期号:3页码:12 |
ISSN号 | 2169-8953 |
关键词 | radiocarbon air-sea CO2 exchange rate seawater bomb C-14 inventory South China sea |
DOI | 10.1029/2021JG006380 |
通讯作者 | Niu, Zhenchuan(niuzc@ieecas.cn) |
英文摘要 | Delta C-14 values of the atmosphere and seawater dissolved inorganic carbon (DIC) were measured during a cruise in the South China Sea (SCS) in September 2015, in order to determine the C-14 flux and bomb C-14-based air-sea CO2 exchange rates for this region. The background atmospheric Delta C-14 value (13.8 +/- 5.0 parts per thousand) for the SCS during that period was lower than that (35.4 +/- 3.4 parts per thousand) of surface seawater (5 m) DIC, and a net transfer of C-14 from the sea to the atmosphere (7.4 +/- 5.0 x 10(11) atoms m(-2) yr(-1)) was determined at the wind speed of 5.2 +/- 1.7 m s(-1). Seawater DIC Delta C-14 profiles showed the highest value (37.9 +/- 3.7 parts per thousand) at a depth of 100 m, a rapid decrease below that depth to -220.3 +/- 3.2 parts per thousand at 1,500 m, and nearly constant values below 1,500 m. The average mean penetration depth of bomb C-14 was 585.5 +/- 99.2 m, and a value of 8.2 +/- 1.0 x 10(9) atoms cm(-2) was obtained for the bomb C-14 inventory in this region. Based on this inventory, a long-term (1954-2015) average air-sea CO2 exchange rate of 20.2 +/- 2.8 mol m(-2) yr(-1) was traced for the SCS. Combined with the pCO(2) measurements in this region, a net CO2 flux rate of 0.54 +/- 0.08 mol m(-2) yr(-1) was yielded for the SCS, which is comparable to the cruise measured flux (0.44 +/- 0.62 mol m(-2) yr(-1)) obtained from a synthesis study (Li et al., 2020, https://doi.org/10.1016/j.pocean.2020.102272). Our study highlights the importance of continued atmospheric and seawater C-14 observations on determining the air-sea flux in this region. |
WOS关键词 | CARBON-DIOXIDE ; TEMPORAL VARIATIONS ; BOMB RADIOCARBON ; SURFACE-WATER ; GAS-EXCHANGE ; WIND-SPEED ; C-14 ; OCEAN ; GEOSECS ; CIRCULATION |
资助项目 | National Natural Science Foundation of China[41773141] ; National Natural Science Foundation of China[42173082] ; National Natural Science Foundation of China[41730108] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA23010302] ; Chinese Academy of Sciences[QYZDY-SSW-DQC001] ; Chinese Academy of Sciences[ZDBS-SSW-DQC001] ; Chinese Academy of Sciences[Y354011480] ; Chinese Academy of Sciences[SKLLQGPY1610] ; Natural Science Basic Research Program of Shaanxi[2019JCW-20] ; Natural Science Foundation of Shaanxi[2014JQ2-4018] |
WOS研究方向 | Environmental Sciences & Ecology ; Geology |
语种 | 英语 |
出版者 | AMER GEOPHYSICAL UNION |
WOS记录号 | WOS:000777487700022 |
资助机构 | National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Chinese Academy of Sciences ; Natural Science Basic Research Program of Shaanxi ; Natural Science Foundation of Shaanxi |
源URL | [http://ir.ieecas.cn/handle/361006/17646] |
专题 | 地球环境研究所_加速器质谱中心 |
通讯作者 | Niu, Zhenchuan |
作者单位 | 1.Xian Inst Innovat Earth Environm Res, Xian, Peoples R China 2.Natl Observat & Res Stn Reg Ecol Environm Change, Xian, Peoples R China 3.Joint Xian AMS Ctr IEECAS & Xian Jiaotong Univ, Shaanxi Prov Key Lab Accelerator Mass Spectrometr, Xian, Peoples R China 4.Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Ocean Continental Climate & Environm, Qingdao, Peoples R China 5.Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Peoples R China |
推荐引用方式 GB/T 7714 | Niu, Zhenchuan,Zhou, Weijian,Zhao, Huiyizhe,et al. Radiocarbon in the Atmosphere and Seawater in the South China Sea: Flux, Inventory and Air-Sea CO2 Exchange Rate Tracing[J]. JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES,2022,127(3):12. |
APA | Niu, Zhenchuan,Zhou, Weijian,Zhao, Huiyizhe,Feng, Xue,&Lyu, Mengni.(2022).Radiocarbon in the Atmosphere and Seawater in the South China Sea: Flux, Inventory and Air-Sea CO2 Exchange Rate Tracing.JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES,127(3),12. |
MLA | Niu, Zhenchuan,et al."Radiocarbon in the Atmosphere and Seawater in the South China Sea: Flux, Inventory and Air-Sea CO2 Exchange Rate Tracing".JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES 127.3(2022):12. |
入库方式: OAI收割
来源:地球环境研究所
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