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CAS IR Grid
机构
金属研究所 [4]
大连化学物理研究所 [3]
广州能源研究所 [3]
青岛生物能源与过程研... [2]
生态环境研究中心 [2]
新疆理化技术研究所 [1]
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OAI收割 [19]
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期刊论文 [19]
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2023 [2]
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2020 [3]
2019 [2]
2018 [3]
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学科主题
物理化学与绿色催化 [1]
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Coordination polymer-derived non-precious metal catalyst for propane dehydrogenation: Highly dispersed zinc anchored on N-doped carbon
期刊论文
OAI收割
APPLIED SURFACE SCIENCE, 2023, 卷号: 607, 页码: 11
作者:
Cao, Tianlong
;
Dai, Xueya
;
Fu, Yu
;
Qi, Wei
  |  
收藏
  |  
浏览/下载:19/0
  |  
提交时间:2023/05/09
Highly dispersed zinc sites
Metal loading
Coordination polymer
Carbon nanosheet
Propane dehydrogenation
Coordination polymer-derived non-precious metal catalyst for propane dehydrogenation: Highly dispersed zinc anchored on N-doped carbon
期刊论文
OAI收割
APPLIED SURFACE SCIENCE, 2023, 卷号: 607, 页码: 11
作者:
Cao, Tianlong
;
Dai, Xueya
;
Fu, Yu
;
Qi, Wei
  |  
收藏
  |  
浏览/下载:18/0
  |  
提交时间:2023/05/09
Highly dispersed zinc sites
Metal loading
Coordination polymer
Carbon nanosheet
Propane dehydrogenation
Silk fibroin derived porous carbon aerogels confined hyperdispersed Rh nanoparticles to achieve electrocatalytic hydrogen evolution under high current density
期刊论文
OAI收割
DIAMOND AND RELATED MATERIALS, 2022, 卷号: 128, 页码: 6
作者:
Lu, Runqing
;
Sam, Daniel Kobina
;
Gong, Shanhe
;
Wang, Wenbo
;
Ge, Dongdong
  |  
收藏
  |  
浏览/下载:2/0
  |  
提交时间:2024/12/03
Carbon aerogel
Highly-dispersed
Hydrogen evolution reaction
Noble metal
Catalytic oleic acid hydrotreating to bio-aviation fuel over highly dispersed Ni/SAPO-11 catalysts prepared by citric acid and ethylene glycol co-assistance impregnation
期刊论文
OAI收割
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2022, 卷号: 10, 期号: 2, 页码: 10
作者:
Yang, Lingmei
;
Luo, Wen
;
Li, Hui Wen
;
Wang, Hai yong
;
Zhang, Aihua
  |  
收藏
  |  
浏览/下载:17/0
  |  
提交时间:2023/11/21
Oleic acid
Hydroisomerization
Highly dispersed
Ni-SAPO-11 catalyst
Ethylene glycol
Mn-doping induced changes in Pt dispersion and PtxMny alloying extent on Pt/Mn-DMSN catalyst with enhanced propane dehydrogenation stability
期刊论文
OAI收割
JOURNAL OF CATALYSIS, 2020, 卷号: 389, 页码: 450-460
作者:
Fan, Xiaoqiang
;
Liu, Dandan
;
Sun, Xiaoying
;
Yu, Xuehua
;
Li, Dong
  |  
收藏
  |  
浏览/下载:18/0
  |  
提交时间:2021/02/02
Propane dehydrogenation
Mn-doping effect
Highly dispersed PtMn alloy sites
Enhanced stability
Mn-doping induced changes in Pt dispersion and PtxMny alloying extent on Pt/Mn-DMSN catalyst with enhanced propane dehydrogenation stability
期刊论文
OAI收割
JOURNAL OF CATALYSIS, 2020, 卷号: 389, 页码: 450-460
作者:
Fan, Xiaoqiang
;
Liu, Dandan
;
Sun, Xiaoying
;
Yu, Xuehua
;
Li, Dong
  |  
收藏
  |  
浏览/下载:17/0
  |  
提交时间:2021/02/02
Propane dehydrogenation
Mn-doping effect
Highly dispersed PtMn alloy sites
Enhanced stability
No pulsed radio emission during a bursting phase of a Galactic magnetar
期刊论文
OAI收割
Nature, 2020, 卷号: 587, 页码: 63-65
作者:
HXMT
  |  
收藏
  |  
浏览/下载:44/0
  |  
提交时间:2022/02/08
Astrophysics - High Energy Astrophysical Phenomena
Abstract: Fast radio bursts (FRBs) are millisecond-duration radio transients of unknown physical origin observed at extragalactic distances
1-3
. It has long been speculated that magnetars are the engine powering repeating bursts from FRB sources
4-13
, but no convincing evidence has been collected so far
14
. Recently, the Galactic magnetar SRG 1935+2154 entered an active phase by emitting intense soft íray bursts
15
. One FRB-like event with two peaks (FRB 200428) and a luminosity slightly lower than the faintest extragalactic FRBs was detected from the source, in association with a soft íray/hard-X-ray flare
18-21
. Here we report an eight-hour targeted radio observational campaign comprising four sessions and assisted by multi-wavelength (optical and hard-X-ray) data. During the third session, 29 soft-íray repeater (SGR) bursts were detected in íray energies. Throughout the observing period, we detected no single dispersed pulsed emission coincident with the arrivals of SGR bursts, but unfortunately we were not observing when the FRB was detected. The non-detection places a fluence upper limit that is eight orders of magnitude lower than the fluence of FRB 200428. Our results suggest that FRB-SGR burst associations are rare. FRBs may be highly relativistic and geometrically beamed, or FRB-like events associated with SGR bursts may have narrow spectra and characteristic frequencies outside the observed band. It is also possible that the physical conditions required to achieve coherent radiation in SGR bursts are difficult to satisfy, and that only under extreme conditions could an FRB be associated with an SGR burst.
Citric-acid-induced mesoporous SAPO-11 loaded with highly dispersed nickel for enhanced hydroisomerization of oleic acid to iso-alkanes
期刊论文
OAI收割
FUEL PROCESSING TECHNOLOGY, 2019, 卷号: 187, 页码: 52-62
作者:
Yang, Lingmei
;
Xing, Shiyou
;
Sun, Hongzhe
;
Miao, Changlin
;
Li, Ming
  |  
收藏
  |  
浏览/下载:24/0
  |  
提交时间:2020/10/29
Citric acid
Highly dispersed Ni
Mesoporous SAPO-11
Hydroisomerization
Oleic acid
食用蔬菜能吸收和积累微塑料
期刊论文
OAI收割
科学通报, 2019, 卷号: 64, 期号: 9, 页码: 928-934
作者:
李连祯
;
周倩
;
尹娜
;
涂晨
;
骆永明
  |  
收藏
  |  
浏览/下载:142/0
  |  
提交时间:2020/06/17
微塑料
生菜
聚苯乙烯微球
吸收
积累
健康风险
microplastics
lettuce
polystyrene microbeads
uptake
accumulation
human health risk
Microplastic (MP, 100 nm-5 mm) may present an attributable risk to ecosystem and human health, and its pollution has become a global environmental concern. Despite a wealth of information on the accumulation of MPs in aquatic species, there is no information on the uptake and accumulation of MPs by higher plants. Terrestrial edible plants are directly exposed to MPs when agricultural soil was applied with organic manure, sewage sludge as fertilizer or plastic mulching. In this paper, the uptake of two sizes of polystyrene (PS) microbeads (0.2 and 1.0 mum) and then their distribution and migration in an edible plant lettuce were firstly investigated based on laboratory experiments. We used fluorescent markers to track PS microbeads in plant tissues and found fluorescence to be a sensitive and reliable detection method. Sections from untreated control lettuce showed no autofluorescence. When roots were treated with fluorescently labeled PS microbeads, the microbeads could be identified by its fluorescence. Our main study investigated the uptake of 0.2 mum beads, as few luminescence signals were observed in lettuce roots for 1.0 mum beads in our experiment. We observed that 0.2 mum fluorescent microbeads were extracellularly trapped in the root cap mucilage (which is a highly hydrated polysaccharide) and a dark green tip (which was typical of lettuce roots exposed to label PS beads) was usually visible to the naked eye. Confocal images revealed that the PS luminescence signals were mainly located in the vascular system and on the cell walls of the cortex tissue of the roots, indicated that the beads passed through the intercellular space via the apoplastic transport system. Once inside the central cylinder, the 0.2 mum PS beads were transferred from the roots to the stems and leaves via the vascular system following the transpiration stream. We also observed that the PS beads adhered to one another and self-assembled systematically into grape-like and (chain) string-like clusters in the intercellular space of the root and stem vascular tissue of lettuce plant. In contrast to the root and stem, PS beads were dispersed in the leaf tissue. Here, for the first time we provide evidence of the adherence, uptake, accumulation, and translocation of submicrometer MPs within an edible plant. Our findings highlight the previously underappreciated human exposure pathway to MPs through the consumption of contaminated crops and emphasize the need for new management strategies to control the release of MPs waste products into the terrestrial environment. Ultimately, the potential impacts of low range sized MPs on food safety of crop plants and human health need to be urgently considered.
C-C Bonds Cleavage of Biomass-Derived Glycerol to Methane and Ethylene Glycol in Aqueous Phase Over Highly Dispersed Ru-Based Catalysts
期刊论文
OAI收割
ASIAN JOURNAL OF ORGANIC CHEMISTRY, 2018, 卷号: 7, 期号: 10, 页码: 2039-2044
作者:
Xu, Jie
;
Huang, Qian-Qian
;
Yu, Wei-Qiang
;
Luo, Xiao-Lin
;
Gao, Jin
  |  
收藏
  |  
浏览/下载:26/0
  |  
提交时间:2019/06/20
carbothermal reduction
highly dispersed Ru NPs
glycerol
hydrogenolysis
C-C bond cleavage